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[汾渭平原吸光性气溶胶的时空分布特征及潜在来源]

[Spatio-temporal Patterns and Potential Sources of Absorbing Aerosols in the Fenwei Plain].

作者信息

Liu Min-Xia, Li Liang, Yu Rui-Xin, Song Jia-Ying, Zhang Guo-Juan, Mu Ruo-Lan, Xu Lu

机构信息

College of Geography and Environmental Science, Northwest Normal University, Lanzhou 730070, China.

出版信息

Huan Jing Ke Xue. 2021 Jun 8;42(6):2634-2647. doi: 10.13227/j.hjkx.202010098.

Abstract

Air quality has gradually improved in many parts of China; however, air pollution is become more severe in the Fenwei Plain. Using OMI/Aura OMAERUV L2 and PM data, spatial autocorrelation analysis and back trajectory modeling were used to explore the spatio-temporal patterns of absorptive aerosols over the Fenwei Plain, and the dominant types, transmission paths, and potential source areas were identified. The main results can be summarized as follows:① Annual mean absorbing aerosol index (AAI) values increased between 2005 and 2019, with high period occurring in 2006, 2013, and 2017, with values exceeding 0.63. Xi'an and Linfen were identified as a 'high-high' cluster, with AAI showing poor spatial stability and a 15.3% increase in area over the past 15 years. In contrast, the area connecting Xi'an and Linfen, which occupies 24.2% of the total area of the region, was identified as a 'low-low' cluster, with a sharp drop of 6.2% in area; ② The Fenwei Plain has high AAI values across a large area in winter, exceeding 0.8 in Linfen and Xi'an, and 91.5% of the study area exceeding 0.6. Values were lower in spring (AAI>0.4) and autumn (AAI>0.3), with the lowest values occurring in summer. The atmospheric diffusion conditions in spring, autumn, and winter are poor, associated with anticyclonic high-pressure events. The observed high AAI values were significantly affected by atmospheric diffusion conditions, temperature, and precipitation; ③ Back trajectory and source contribution modeling showed that long-range transport of air masses from Xi'an and Linfen occurs from the northwest, and short-range transport air masses occurs from the east and south. Two long-range sand and dust source areas were determined (with northwestern and northern wind sources); two carbon source areas were identified (with eastern and southern wind sources); and one combined sand and carbon source area was identified (from the Loess Plateau). Of these sources, the northwestern wind source, the Loess Plateau, and the southern wind source have significant influence in Xi'an, and the eastern wind source and the Loess Plateau have a significant impact on Linfen. Linfen is little affected by the northwestern wind source and the dust from the northern wind source. Based on the spatial distribution of CO and its correlation with AAI, it is concluded that cardon in the dominant absorbent aerosol in Linfen dust and carbon are most important in Xi'an.

摘要

中国许多地区的空气质量已逐渐改善;然而,汾渭平原的空气污染却日益严重。利用OMI/Aura OMAERUV L2和PM数据,采用空间自相关分析和后向轨迹模型,探讨了汾渭平原吸收性气溶胶的时空分布特征,确定了其主要类型、传输路径和潜在源区。主要结果如下:①2005年至2019年期间,年平均吸收气溶胶指数(AAI)值呈上升趋势,2006年、2013年和2017年出现高值期,值超过0.63。西安和临汾被确定为“高高”聚类,AAI空间稳定性较差,过去15年面积增加了15.3%。相比之下,连接西安和临汾的区域(占该地区总面积的24.2%)被确定为“低低”聚类,面积急剧下降了6.2%;②汾渭平原冬季大面积地区AAI值较高,临汾和西安超过0.8,研究区域91.5%超过0.6。春季(AAI>0.4)和秋季(AAI>0.3)的值较低,夏季最低。春、秋、冬三季大气扩散条件较差,与反气旋高压事件有关。观测到的高AAI值受大气扩散条件、温度和降水的显著影响;③后向轨迹和源贡献模型表明,来自西安和临汾的气团长距离传输来自西北方向,短距离传输气团来自东部和南部。确定了两个长距离沙尘源区(西北风和北风源);确定了两个碳源区(东风和南风源);确定了一个沙尘和碳混合源区(来自黄土高原)。在这些源中,西北风源、黄土高原和南风源对西安影响显著,东风源和黄土高原对临汾影响显著。临汾受西北风源和北风源沙尘的影响较小。基于CO的空间分布及其与AAI的相关性,得出结论:临汾沙尘中占主导地位的吸收性气溶胶中的碳以及西安的碳最为重要。

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