Liu Wei-Jie, Hu Tian-Peng, Mao Yao, Xu An, Su Ye-Wang, Li Xing-Yu, Cheng Cheng, Shi Ming-Ming, Liang Li-Li, Xing Xin-Li, Zhang Jia-Quan, Qi Shi-Hua
School of Environmental Studies, China University of Geosciences, Wuhan 430074, China.
Hubei Key Laboratory of Mine Environmental Pollution Control and Remediation, School of Environmental Science and Engineering, Hubei Polytechnic University, Huangshi 435003, China.
Huan Jing Ke Xue. 2021 Nov 8;42(11):5122-5130. doi: 10.13227/j.hjkx.202101238.
In recent years, frequent haze episodes have resulted in the deterioration of air quality of the Fenwei Plain during winter and holidays. Besides coal combustion and industrial emissions, the topography and climate of the Fenwei Plain were also the main causes of the haze. The samples were collected in Linfen of Fenwei Plain during the Spring Festival from February 2 to February 13, 2019. The 13 elements(Li, Be, Ti, Rb, Sc, Y, La, Ce, Zr, V, Tl, U, and Sn) in PM were determined by inductively coupled plasma mass spectrometry(ICP-MS). Combined with the meteorological data, the spatial and temporal distribution of pollutants and potential source analysis were evaluated by cluster analysis and backward trajectory. The average concentration of SO was 58.39 μg·m during the sampling period, which exceeded the 24 h average mass concentration limit(50.00 μg·m) of national ambient air quality standard(GB 3095-2012). The average concentrations of O, NO, and CO was 52.15 μg·m, 29.02 μg·m, and 2.29 mg·m, respectively. The results showed that SO was the dominated pollutant. NO and CO were mainly affected by diffusion from urban areas. The backward trajectory analysis indicated that the basin topography of the Fenwei Plain may be the main cause of the haze. The analysis of potential source contribution function(PSCF) of soil sources showed that the potential dominated areas included Northern Shaanxi, southern Gansu and Southern Ningxia., which were mainly affected by the monsoon climate.
近年来,频繁的雾霾天气导致汾渭平原冬季和节假日期间空气质量恶化。除了煤炭燃烧和工业排放外,汾渭平原的地形和气候也是雾霾的主要成因。于2019年2月2日至13日春节期间在汾渭平原的临汾采集样本。采用电感耦合等离子体质谱法(ICP-MS)测定了PM中的13种元素(锂、铍、钛、铷、钪、钇、镧、铈、锆、钒、铊、铀和锡)。结合气象数据,通过聚类分析和后向轨迹法对污染物的时空分布及潜在源进行了分析。采样期间SO的平均浓度为58.39μg·m,超过了国家环境空气质量标准(GB 3095-2012)的24小时平均质量浓度限值(50.00μg·m)。O、NO和CO的平均浓度分别为52.