Kim Chan, Scholz Markus, Madsen Anders
European X-ray Free-Electron Laser Facility, Holzkoppel 4, 22869 Schenefeld, Germany.
J Synchrotron Radiat. 2021 Jul 1;28(Pt 4):1159-1165. doi: 10.1107/S160057752100477X. Epub 2021 Jun 1.
A quantitative analysis of the effect of strain on phase retrieval in Bragg coherent X-ray diffraction imaging is reported. It is shown in reconstruction simulations that the phase maps of objects with strong step-like phase changes are more precisely retrieved than the corresponding modulus values. The simulations suggest that the reconstruction precision for both phase and modulus can be improved by employing a modulus homogenization (MH) constraint. This approach was tested on experimental data from a highly strained Fe-Al crystal which also features antiphase domain boundaries yielding characteristic π phase shifts of the (001) superlattice reflection. The impact of MH is significant and this study outlines a successful method towards imaging of strong phase objects using the next generation of coherent X-ray sources, including X-ray free-electron lasers.
报道了对布拉格相干X射线衍射成像中应变对相位恢复影响的定量分析。重建模拟表明,具有强烈阶梯状相位变化的物体的相位图比相应的模量值能更精确地恢复。模拟表明,通过采用模量均匀化(MH)约束可以提高相位和模量的重建精度。该方法在来自高应变铁铝晶体的实验数据上进行了测试,该晶体还具有反相畴界,产生(001)超晶格反射的特征π相移。MH的影响显著,本研究概述了一种使用包括X射线自由电子激光在内的下一代相干X射线源对强相位物体进行成像的成功方法。