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沿南水北调东线工程蓄水水库的优先污染物筛选的环境影响。

Environmental implications from the priority pollutants screening in impoundment reservoir along the eastern route of China's South-to-North Water Diversion Project.

机构信息

State Key Laboratory of Lake Science and Environment Research, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China.

State Key Laboratory of Lake Science and Environment Research, Nanjing Institute of Geography and Limnology, Chinese Academy of Sciences, Nanjing 210008, China; University of Chinese Academy of Sciences, Beijing 100049, China.

出版信息

Sci Total Environ. 2021 Nov 10;794:148700. doi: 10.1016/j.scitotenv.2021.148700. Epub 2021 Jun 25.

Abstract

Screening priority pollutants from vast anthropogenic contaminants discharged into aquatic environment is urgent for protecting water quality definitely. The multi-criteria scoring method involved in the occurrence (O), persistence (P), bioaccumulation (B), ecological risk (Eco-T), and human health risk (Hum-T), was established for pollutants prioritization in waters and applied in Dongping Lake, the final impoundment reservoir along the eastern route of China's South-to-North Water Diversion Project (SNWDP). A total of 170 chemicals including heavy metals (HMs), volatile organic chemicals (VOCs), polycyclic aromatic hydrocarbons (PAHs), organochlorine pesticides (OCPs), polychlorinated biphenyls (PCBs), phthalate esters (PAEs), and antibiotics (ANTs) were investigated as the candidates. Accordingly, 42 chemicals including 8 PAEs, 7 OCPs, 7 PCBs, 5 PAHs, 13 HMs, and 2 VOCs were made up the list of priority pollutants for Dongping Lake, suggesting the necessity of routine monitoring high priority groups and revising the existing list. Multiple risk assessment indicated higher ecological and human health risks induced by HMs than by organic pollutants. Spatial distribution of risks stressed the retention of toxic organic chemicals by the lake body and the accumulation of HMs along the transfer route, respectively, thus triggering ecosystem responses and potential effects on the water-receiving areas as expected.

摘要

筛选排入水生环境的大量人为污染物中的优先污染物对于明确保护水质至关重要。本研究建立了涉及污染物在水中出现(Occurrence,O)、持久性(Persistence,P)、生物累积性(Bioaccumulation,B)、生态风险(Ecological Risk,Eco-T)和人体健康风险(Human Health Risk,Hum-T)的多标准评分方法,并将其应用于中国南水北调东线工程最后一座调蓄水库——东平湖。共调查了 170 种化学物质,包括重金属(HMs)、挥发性有机化合物(VOCs)、多环芳烃(PAHs)、有机氯农药(OCPs)、多氯联苯(PCBs)、邻苯二甲酸酯(PAEs)和抗生素(ANTs)等,作为候选污染物。因此,包括 8 种邻苯二甲酸酯、7 种有机氯农药、7 种多氯联苯、5 种多环芳烃、13 种重金属和 2 种挥发性有机化合物在内的 42 种化学物质被列为东平湖优先污染物,这表明有必要对高优先群体进行常规监测,并修订现有的清单。多项风险评估表明,重金属引起的生态和人体健康风险高于有机污染物。风险的空间分布分别强调了湖体对有毒有机化学物质的截留作用和沿传输路径对重金属的积累作用,从而引发了预期的生态系统响应和对受水区的潜在影响。

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