Barrer Centre, Department of Chemical Engineering, Imperial College London, London SW7 2AZ, U.K.
Centre for Environmental Policy, Imperial College London, London SW7 1NE, U.K.
Environ Sci Technol. 2021 Aug 3;55(15):10619-10632. doi: 10.1021/acs.est.0c07261. Epub 2021 Jul 9.
As more countries commit to a net-zero GHG emission target, we need a whole energy and industrial system approach to decarbonization rather than focus on individual emitters. This paper presents a techno-economic analysis of monoethanolamine-based post-combustion capture to explore opportunities over a diverse range of power and industrial applications. The following ranges were investigated: feed gas flow rate between 1-1000 kg ·s, gas CO concentrations of 2-42%, capture rates of 70-99%, and interest rates of 2-20%. The economies of scale are evident when the flue gas flow rate is <20 kg ·s and gas concentration is below 20% CO. In most cases, increasing the capture rate from 90 to 95% has a negligible impact on capture cost, thereby reducing CO emissions at virtually no additional cost. The majority of the investigated space has an operating cost fraction above 50%. In these instances, reducing the cost of capital (, interest rate) has a minor impact on the capture cost. Instead, it would be more beneficial to reduce steam requirements. We also provide a surrogate model which can evaluate capture cost from inputs of the gas flow rate, CO composition, capture rate, interest rate, steam cost, and electricity cost.
随着越来越多的国家承诺实现温室气体净零排放目标,我们需要采取整体能源和工业系统方法来实现脱碳,而不是仅仅关注个别排放者。本文对基于一乙醇胺的燃烧后捕集技术进行了技术经济分析,以探索在各种电力和工业应用中的机会。研究范围如下:进气流量在 1-1000kg·s 之间,气体 CO 浓度为 2-42%,捕集率为 70-99%,利率为 2-20%。当烟气流量<20kg·s 且气体浓度低于 20%CO 时,规模经济效应明显。在大多数情况下,将捕集率从 90%提高到 95%对捕集成本几乎没有影响,从而在几乎不增加成本的情况下减少 CO 排放。在所研究的大部分空间中,运行成本占比超过 50%。在这些情况下,降低资本成本(利率)对捕集成本的影响较小。相反,减少蒸汽需求将更有益。我们还提供了一个替代模型,可以根据气体流量、CO 组成、捕集率、利率、蒸汽成本和电力成本等输入来评估捕集成本。