VIB Center for Inflammation Research, 9052, Ghent, Belgium.
Department of Biomedical Molecular Biology, Ghent University, 9052, Ghent, Belgium.
Cell Death Dis. 2021 Jul 14;12(7):699. doi: 10.1038/s41419-021-03994-0.
Butylate hydroxyanisole (BHA) is a synthetic phenol that is widely utilized as a preservative by the food and cosmetic industries. The antioxidant properties of BHA are also frequently used by scientists to claim the implication of reactive oxygen species (ROS) in various cellular processes, including cell death. We report on the surprising finding that BHA functions as a direct inhibitor of RIPK1, a major signaling hub downstream of several immune receptors. Our in silico analysis predicts binding of 3-BHA, but not 2-BHA, to RIPK1 in an inactive DLG-out/Glu-out conformation, similar to the binding of the type III inhibitor Nec-1s to RIPK1. This predicted superior inhibitory capacity of 3-BHA over 2-BHA was confirmed in cells and using in vitro kinase assays. We demonstrate that the reported protective effect of BHA against tumor necrosis factor (TNF)-induced necroptotic death does not originate from ROS scavenging but instead from direct RIPK1 enzymatic inhibition, a finding that most probably extends to other reported effects of BHA. Accordingly, we show that BHA not only protects cells against RIPK1-mediated necroptosis but also against RIPK1 kinase-dependent apoptosis. We found that BHA treatment completely inhibits basal and induced RIPK1 enzymatic activity in cells, monitored at the level of TNFR1 complex I under apoptotic conditions or in the cytosol under necroptosis. Finally, we show that oral administration of BHA protects mice from RIPK1 kinase-dependent lethality caused by TNF injection, a model of systemic inflammatory response syndrome. In conclusion, our results demonstrate that BHA can no longer be used as a strict antioxidant and that new functions of RIPK1 may emerge from previously reported effects of BHA.
丁羟茴醚(BHA)是一种人工合成的酚类物质,被广泛应用于食品和化妆品行业作为防腐剂。BHA 的抗氧化特性也经常被科学家用于声称活性氧物种(ROS)在各种细胞过程中的作用,包括细胞死亡。我们报告了一个令人惊讶的发现,BHA 作为 RIPK1 的直接抑制剂发挥作用,RIPK1 是几种免疫受体下游的主要信号枢纽。我们的计算机分析预测,3-BHA 而不是 2-BHA 与 RIPK1 结合,处于非活性的 DLG-out/Glu-out 构象,类似于 III 型抑制剂 Nec-1s 与 RIPK1 的结合。这种预测的 3-BHA 比 2-BHA 具有更高的抑制能力,在细胞中和使用体外激酶测定中得到了证实。我们证明,BHA 对抗肿瘤坏死因子(TNF)诱导的坏死性细胞死亡的保护作用不是来自于 ROS 清除,而是来自于 RIPK1 的直接酶抑制,这一发现很可能扩展到 BHA 的其他报道的作用。因此,我们表明 BHA 不仅可以保护细胞免受 RIPK1 介导的坏死,还可以防止 RIPK1 激酶依赖性凋亡。我们发现,BHA 处理完全抑制了细胞中基础和诱导的 RIPK1 酶活性,在凋亡条件下通过 TNFR1 复合物 I 或在坏死时通过细胞质进行监测。最后,我们表明,BHA 的口服给药可保护小鼠免受 TNF 注射引起的 RIPK1 激酶依赖性致死,这是全身炎症反应综合征的模型。总之,我们的结果表明,BHA 不能再被用作严格的抗氧化剂,并且 RIPK1 的新功能可能会从 BHA 的先前报道的作用中出现。