Yang Xianguang, Wen Long, Yan Jiahao, Bao Yanjun, Chen Qin, Camposeo Andrea, Pisignano Dario, Li Baojun
Institute of Nanophotonics, Jinan University, Guangzhou 511443, China.
NEST, Istituto Nanoscienze-CNR and Scuola Normale Superiore, Piazza S. Silvestro 12, I-56127 Pisa, Italy.
J Phys Chem Lett. 2021 Jul 29;12(29):7034-7040. doi: 10.1021/acs.jpclett.1c01690. Epub 2021 Jul 21.
The delivery of optical signals from an external light source to a nanoscale waveguide is highly important for the development of nanophotonic circuits. However, the efficient coupling of external light energy into nanophotonic components is difficult and still remains a challenge. Herein, we use an external silica nanofiber to light up an organic-inorganic hybrid nanowaveguide, namely, a system composed of a polymer filament doped with MoS quantum dots. Nanofiber-excited nanowaveguides in a crossed geometry are found to asymmetrically couple excitation signals along two opposite directions, with different energy dissipation resulting in different colors of the light emitted by MoS quantum dots and collected from the waveguide terminals. Interestingly, rainbow-like light in the hybrid waveguide is achieved by three-in-one mixing of red, green, and blue components. This heterodimensional system of dots in waveguide represents a significant advance toward all-optical routing and full-color display in integrated nanophotonic devices.
将光信号从外部光源传输到纳米级波导对于纳米光子电路的发展至关重要。然而,将外部光能有效耦合到纳米光子组件中是困难的,并且仍然是一个挑战。在此,我们使用外部二氧化硅纳米纤维来点亮有机-无机杂化纳米波导,即由掺杂有MoS量子点的聚合物细丝组成的系统。发现交叉几何结构中的纳米纤维激发纳米波导沿两个相反方向不对称地耦合激发信号,不同的能量耗散导致MoS量子点发射并从波导终端收集的光有不同颜色。有趣的是,通过红、绿、蓝分量的三合一混合在混合波导中实现了彩虹般的光。这种波导中量子点的异维系统代表了集成纳米光子器件在全光路由和全彩显示方面的重大进展。