High Accuracy Ultrafast Spatiotemporal Pump-Probe Measurement of Electrical Thermal Transport in Thin Film Gold.

A high resolution spatiotemporal ultrafast pump-probe system is developed to examine the interactions and transport phenomena between the electrical and the lattice thermal subsystems during ultrafast laser-matter interactions. This system incorporates an ultrafast pump-probe scheme with a stationary probe beam that interrogates the response to a spatial scanning pump beam, providing a full spatiotemporal mapping of a material's response due to an ultrafast pump excitation. The material's response, which is highly sensitive to its transport properties, is measured with a high spatial accuracy of up to ±10 nm and subpicosecond time resolution. Details of achieving this high spatial accuracy are described, and a study of the ultrafast transport processes in thin film gold is demonstrated. With the aid of transport and optical response models, the electrical thermal transport properties of gold and the electron-lattice coupling constant are simultaneously determined.