NTNU Nanomechanical Lab, Department of Structural Engineering, Norwegian University of Science and Technology (NTNU), Trondheim, 7491, Norway.
College of Materials and Environmental Engineering, Hangzhou Dianzi University, Hangzhou, 310018, China.
Adv Sci (Weinh). 2021 Nov;8(21):e2101163. doi: 10.1002/advs.202101163. Epub 2021 Sep 9.
Remarkable progress has been made in surface icephobicity in the recent years. The mainstream standpoint of the reported antiicing surfaces yet only considers the ice-substrate interface and its adjacent regions being of static nature. In reality, the local structures and the overall properties of ice-substrate interfaces evolve with time, temperature and various external stimuli. Understanding the dynamic properties of the icing interface is crucial for shedding new light on the design of new anti-icing surfaces to meet challenges of harsh conditions including extremely low temperature and/or long working time. This article surveys the state-of-the-art anti-icing surfaces and dissects their dynamic changes of the chemical/physical states at icing interface. According to the focused critical ice-substrate contacting locations, namely the most important ice-substrate interface and the adjacent regions in the substrate and in the ice, the available anti-icing surfaces are for the first time re-assessed by taking the dynamic evolution into account. Subsequently, the recent works in the preparation of dynamic anti-icing surfaces (DAIS) that consider time-evolving properties, with their potentials in practical applications, and the challenges confronted are summarized and discussed, aiming for providing a thorough review of the promising concept of DAIS for guiding the future icephobic materials designs.
近年来,在表面抗冰性方面取得了显著进展。然而,报道的抗冰表面的主流观点仅考虑了冰-基底界面及其相邻区域处于静态性质。实际上,冰-基底界面的局部结构和整体性质随时间、温度和各种外部刺激而演变。了解冰界面的动态特性对于揭示新的抗冰表面设计至关重要,以应对包括极低温度和/或长时间工作在内的恶劣条件的挑战。本文综述了最新的抗冰表面,并剖析了它们在冰界面处化学/物理状态的动态变化。根据聚焦的关键冰-基底接触位置,即最重要的冰-基底界面以及基底和冰中的相邻区域,首次考虑动态演变重新评估了现有的抗冰表面。随后,总结和讨论了考虑时间演变特性的动态抗冰表面(DAIS)的最新制备工作,及其在实际应用中的潜力,以及面临的挑战,旨在为 DAIS 的有前途的概念提供全面的综述,以指导未来的冰斥材料设计。