Gao Yuechen, Zhu Xi
School of Science and Engineering (SSE), CUHK-Shenzhen Shenzhen Institute of Artificial Intelligence and Robotics for Society (AIRS), Longgang District, Shenzhen, Guangdong 518172, China.
J Phys Chem Lett. 2021 Sep 23;12(37):9124-9131. doi: 10.1021/acs.jpclett.1c02486. Epub 2021 Sep 15.
The magic-angle twisted bilayer graphene (MATBG) recently attracted intensive research attention because of its fascinating and unconventional electronic properties. Herein, we claim the magic-angle phenomenon originates from the Heisenberg uncertainty principle, which can provide intensive explanations on finite size effect and twist-dependent low energy band variations. We showed that flat bands could exist only near the AA stacking structure rather than AB. The finite-size effect gives the minimal size of graphene quantum dots ( ≳ 4 nm) for the emergence of the Dirac point, and the uncertainty relation provides the upper bound for moiré supercells ( ≲ 23.5 nm) in twisted bilayer graphene, which is the quantum mechanical boundary for the emergence of flat bands. Combining the twist dependence of moiré supercell size, we proved that there is only one possible magic angle in MATBG at θ ≈ 1.1°. Our result implies that the unconventional phenomena in MATBG originate from the fundamental feature of condensed matter physics.
魔角扭曲双层石墨烯(MATBG)因其迷人且非常规的电子特性,最近吸引了广泛的研究关注。在此,我们声称魔角现象源于海森堡不确定性原理,该原理能够对有限尺寸效应和与扭曲相关的低能带变化给出详尽解释。我们表明,平带仅能出现在AA堆垛结构附近,而非AB堆垛结构。有限尺寸效应给出了石墨烯量子点出现狄拉克点的最小尺寸(≳4纳米),并且不确定性关系给出了扭曲双层石墨烯中莫尔超胞的上限(≲23.5纳米),这是平带出现的量子力学边界。结合莫尔超胞尺寸的扭曲依赖性,我们证明了在MATBG中,仅在θ≈1.1°时存在一个可能的魔角。我们的结果表明,MATBG中的非常规现象源于凝聚态物理的基本特征。