Peřina Jan, Michálek Václav, Machulka Radek, Haderka Ondřej
Opt Express. 2021 Sep 13;29(19):29704-29719. doi: 10.1364/OE.431204.
Photon-number-resolved post-selection on one beam out of a correlated system of three beams with bi-partite photon-number correlations gives rise to joint photon-number distributions with the probabilities forming checkered patterns. These patterns originate in the convolution of two constituting photon-number distributions, one endowed with correlations in photon numbers, the other exhibiting anti-correlations in photon-number fluctuations. Using three twin beams of comparable intensity whose constituting beams suitably overlap on the photocathode of a photon-number-resolving iCCD camera, we experimentally as well as theoretically analyze the properties of such states as they change with the varying ratio of the correlated and anti-correlated contributions. The experimental photocount 2D histograms of the fields post-selected by the iCCD camera that are reconstructed by the maximum-likelihood approach confirm their non-classicality though the limited detection efficiency in post-selection conceals the checkered patterns. Contrary to this, the maximum-likelihood reconstruction of the experimental 3D photocount histogram similarly as a suitable 3D Gaussian fit, that reveal the states as they would be obtained by ideal post-selection, provide the photon-number distributions with the checkered patterns. The corresponding quasi-distributions of integrated intensities are determined. Nonclassical properties of the generated states are investigated using suitable non-classicality criteria and the corresponding non-classicality depths. These states with their correlations of varying intensity are prospective for two-photon excitations of atoms and molecules as well as two-photon spectroscopy.
在具有二分光子数关联的三束光的相关系统中,对其中一束光进行光子数分辨后选择,会产生联合光子数分布,其概率形成棋盘图案。这些图案源于两个构成光子数分布的卷积,一个在光子数上具有关联,另一个在光子数涨落上表现出反关联。使用三束强度相当的孪生光束,其构成光束在光子数分辨型增强电荷耦合器件(iCCD)相机的光电阴极上适当重叠,我们通过实验和理论分析了这些态的性质随关联和反关联贡献的变化比例如何改变。iCCD相机后选择的场的实验光计数二维直方图通过最大似然法重建,证实了它们的非经典性,尽管后选择中的有限检测效率掩盖了棋盘图案。与此相反,实验三维光计数直方图的最大似然重建以及合适的三维高斯拟合,揭示了理想后选择时所获得的态,给出了具有棋盘图案的光子数分布。确定了相应的积分强度准分布。使用合适的非经典性判据和相应的非经典性深度研究了所产生态的非经典性质。这些具有不同强度关联的态在原子和分子的双光子激发以及双光子光谱学方面具有前景。