Zhang Jing, Yang Zhilong, Liu Shuai, Xia Wei, Zhu Tongshuai, Chen Cheng, Wang Chengwei, Wang Meixiao, Mo Sung-Kwan, Yang Lexian, Kou Xufeng, Guo Yanfeng, Zhang Haijun, Liu Zhongkai, Chen Yulin
School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.
University of Chinese Academy of Sciences, Beijing 100049, China.
ACS Nano. 2021 Oct 26;15(10):15850-15857. doi: 10.1021/acsnano.1c03666. Epub 2021 Oct 13.
Quantum well states (QWSs) can form at the surface or interfaces of materials with confinement potential. They have broad applications in electronic and optical devices such as high mobility electron transistor, photodetector, and quantum well laser. The properties of the QWSs are usually the key factors for the performance of the devices. However, direct visualization and manipulation of such states are, in general, challenging. In this work, by using angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling microscopy/spectroscopy (STM/STS), we directly probe the QWSs generated on the vacuum interface of a narrow band gap semiconductor NbSiTe. Interestingly, the position and splitting of QWSs could be easily manipulated via potassium (K) dosage onto the sample surface. Our results suggest NbSiTe to be an intriguing semiconductor system to study and engineer the QWSs, which has great potential in device applications.
量子阱态(QWSs)可在具有限制势的材料表面或界面形成。它们在诸如高迁移率电子晶体管、光电探测器和量子阱激光器等电子和光学器件中有着广泛应用。量子阱态的性质通常是器件性能的关键因素。然而,一般来说,直接可视化和操控这些态具有挑战性。在这项工作中,通过使用角分辨光电子能谱(ARPES)和扫描隧道显微镜/能谱(STM/STS),我们直接探测了窄带隙半导体NbSiTe真空界面上产生的量子阱态。有趣的是,通过向样品表面施加钾(K)剂量,可以轻松操控量子阱态的位置和分裂。我们的结果表明NbSiTe是一个用于研究和设计量子阱态的有趣半导体系统,在器件应用方面具有巨大潜力。