Du Chenjun, Guo Qingjun, Zhang Jun
Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China; University of Chinese Academy of Sciences, Beijing 100049, China.
Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing 100101, China.
Sci Total Environ. 2022 Feb 1;806(Pt 4):150765. doi: 10.1016/j.scitotenv.2021.150765. Epub 2021 Oct 16.
Moss nitrogen (N) concentration and isotopic composition (δN) values can reveal a better understanding of atmospheric N deposition patterns. Here, we summarize the moss N content and δN signatures using data compiled from 104 papers. Based on the dataset, we summarize the models for assessing the level and reduced (NH): oxidised compounds (NO) ratio of atmospheric N deposition. Results showed a historical increase in N concentration and N depletion of specimen mosses close to anthropogenic N sources from intensive animal production and agricultural activities (NH emission) since the 1800s. However, an increase of moss N with a less negative N observed in the last three decades could be due to a substantial fossil fuel combustion contributed NO emission. Spatially, N deposition in Europe decreased due to successful control actions, but Asia has become a hotspot for NH emission from agriculture. The present results highlight the importance of moss N and δN values for estimating atmospheric N deposition patterns at spatio-temporal trends.
苔藓中的氮(N)浓度和同位素组成(δN)值有助于更深入地了解大气氮沉降模式。在此,我们利用从104篇论文中收集的数据总结了苔藓的氮含量和δN特征。基于该数据集,我们总结了评估大气氮沉降水平以及还原态(NH)与氧化态化合物(NO)比例的模型。结果表明,自19世纪以来,靠近来自集约化畜牧生产和农业活动(NH排放)的人为氮源的苔藓标本中的氮浓度呈历史性增加,且氮出现贫化。然而,在过去三十年中观察到苔藓氮增加且氮的负值减小,这可能是由于大量化石燃料燃烧导致的NO排放。在空间上,由于成功的控制措施,欧洲的氮沉降有所减少,但亚洲已成为农业NH排放的热点地区。目前的结果凸显了苔藓氮和δN值对于估算时空趋势下大气氮沉降模式的重要性。