Edelstein Shulamit, García-Martín Antonio, Serena Pedro A, Marqués Manuel I
Instituto de Ciencia de Materiales de Madrid (ICMM-CSIC), Campus de Cantoblanco, 28049, Madrid, Spain.
Instituto de Micro y Nanotecnología IMN-CNM, CSIC, CEI UAM+CSIC, Isaac Newton 8, Tres Cantos, 28760, Madrid, Spain.
Sci Rep. 2021 Oct 21;11(1):20820. doi: 10.1038/s41598-021-00217-6.
In this paper we show analytically and numerically the formation of a near-field stable optical binding between two identical plasmonic particles, induced by an incident plane wave. The equilibrium binding distance is controlled by the angle between the polarization plane of the incoming field and the dimer axis, for which we have calculated an explicit formula. We have found that the condition to achieve stable binding depends on the particle's dielectric function and happens near the frequency of the dipole plasmonic resonance. The binding stiffness of this stable attaching interaction is four orders of magnitude larger than the usual far-field optical binding and is formed orthogonal to the propagation direction of the incident beam (transverse binding). The binding distance can be further manipulated considering the magneto-optical effect and an equation relating the desired equilibrium distance with the required external magnetic field is obtained. Finally, the effect induced by the proposed binding method is tested using molecular dynamics simulations. Our study paves the way to achieve complete control of near-field binding forces between plasmonic nanoparticles.
在本文中,我们通过解析和数值方法展示了由入射平面波诱导的两个相同等离子体粒子之间近场稳定光学束缚的形成。平衡束缚距离由入射场的偏振平面与二聚体轴之间的夹角控制,我们为此计算了一个明确的公式。我们发现实现稳定束缚的条件取决于粒子的介电函数,并且发生在偶极等离子体共振频率附近。这种稳定附着相互作用的束缚刚度比通常的远场光学束缚大四个数量级,并且与入射光束的传播方向正交形成(横向束缚)。考虑磁光效应可以进一步控制束缚距离,并得到了将所需平衡距离与所需外部磁场相关联的方程。最后,使用分子动力学模拟测试了所提出的束缚方法所诱导的效应。我们的研究为实现对等离激元纳米粒子之间近场束缚力的完全控制铺平了道路。