Cao Bo-Wen, Li Cheng, Shi Wei-Jie, Han Cai-Qin, Wu Ying, Yan Chang-Chun
Opt Express. 2021 Oct 11;29(21):34427-34440. doi: 10.1364/OE.440535.
A large-area mid-infrared broadband absorber is proposed in this paper. The absorber is a spiral ITO structure grown on a hexagonal lattice arrangement of silicon nanopillars by using a glancing angle deposition method. The experimental results show that when the heights of the silicon nanopillars are 1.7 µm and the number of rotation depositions is n = 5, that is, the rotation angle is 150 degrees, the absorber absorbs more than 81% of electromagnetic waves in the 2.5-6 µm spectral range. In the atmospheric window of 3-5 µm, the integral absorption reaches 96%. The experimental results also show that the absorbing ability of the ITO structure in the mid-infrared atmospheric window is significantly stronger than that of the structure composed of silver under the same preparation conditions. The main reasons for the broadband absorption are that the spiral ITO structure has resonant absorption of electromagnetic waves with different wavelengths in the empty cavity regions with different sizes, and ITO has longer penetration depths than noble metals in the mid-infrared band, which brings about stronger broadband absorption. The combination of the two leads to a broadening of the total absorption spectrum. The higher heights of the silicon nanopillars enhance absorption further. Additionally, the loose spiral ITO distributions indicate lower mean plasma concentration and then increase penetration depths further, resulting in stronger light absorption. Such a large-area mid-infrared absorption structure with a simple preparation method has potential applications in mid-infrared cloaking and sensing.
本文提出了一种大面积中红外宽带吸收器。该吸收器是一种通过掠角沉积法生长在硅纳米柱六边形晶格排列上的螺旋ITO结构。实验结果表明,当硅纳米柱的高度为1.7μm且旋转沉积次数n = 5,即旋转角度为150度时,该吸收器在2.5 - 6μm光谱范围内吸收超过81%的电磁波。在3 - 5μm的大气窗口中,积分吸收率达到96%。实验结果还表明,在相同制备条件下,ITO结构在中红外大气窗口的吸收能力明显强于由银组成的结构。宽带吸收的主要原因是螺旋ITO结构在不同尺寸的空腔区域对不同波长的电磁波具有共振吸收,并且ITO在中红外波段比贵金属具有更长的穿透深度,这带来了更强的宽带吸收。两者的结合导致总吸收光谱变宽。硅纳米柱更高的高度进一步增强了吸收。此外,松散的螺旋ITO分布表明平均等离子体浓度较低,进而进一步增加穿透深度,导致更强的光吸收。这种制备方法简单的大面积中红外吸收结构在中红外隐身和传感方面具有潜在应用。