Skruszewicz S, Przystawik A, Schwickert D, Sumfleth M, Namboodiri M, Hilbert V, Klas R, Gierschke P, Schuster V, Vorobiov A, Haunhorst C, Kip D, Limpert J, Rothhardt J, Laarmann T
Opt Express. 2021 Nov 22;29(24):40333-40344. doi: 10.1364/OE.446563.
Short-pulse metrology and dynamic studies in the extreme ultraviolet (XUV) spectral range greatly benefit from interferometric measurements. In this contribution a Michelson-type all-reflective split-and-delay autocorrelator operating in a quasi amplitude splitting mode is presented. The autocorrelator works under a grazing incidence angle in a broad spectral range (10 nm - 1 μm) providing collinear propagation of both pulse replicas and thus a constant phase difference across the beam profile. The compact instrument allows for XUV pulse autocorrelation measurements in the time domain with a single-digit attosecond precision and a useful scan length of about 1 ps enabling a decent resolution of E/ΔE = 2000 at 26.6 eV. Its performance for selected spectroscopic applications requiring moderate resolution at short wavelengths is demonstrated by characterizing a sharp electronic transition at 26.6 eV in Ar gas. The absorption of the 11 harmonic of a frequency-doubled Yb-fiber laser leads to the well-known 3s3p4pP Fano resonance of Ar atoms. We benchmark our time-domain interferometry results with a high-resolution XUV grating spectrometer and find an excellent agreement. The common-path interferometer opens up new opportunities for short-wavelength femtosecond and attosecond pulse metrology and dynamic studies on extreme time scales in various research fields.
在极紫外(XUV)光谱范围内的短脉冲计量学和动力学研究极大地受益于干涉测量。在本论文中,我们介绍了一种工作在准振幅分割模式下的迈克尔逊型全反射分束延迟自相关仪。该自相关仪在宽光谱范围(10纳米 - 1微米)内以掠入射角工作,能使两个脉冲复制品共线传播,从而在光束轮廓上提供恒定的相位差。这种紧凑的仪器能够在时域中以个位数阿秒的精度进行XUV脉冲自相关测量,其有效扫描长度约为1皮秒,在26.6电子伏特时能实现E/ΔE = 2000的良好分辨率。通过对氩气中26.6电子伏特处的尖锐电子跃迁进行表征,展示了其在需要短波长中等分辨率的选定光谱应用中的性能。倍频镱光纤激光器的11次谐波的吸收导致了氩原子众所周知的3s3p4pP法诺共振。我们将时域干涉测量结果与高分辨率XUV光栅光谱仪进行了基准测试,发现二者吻合度极佳。这种共光路干涉仪为短波长飞秒和阿秒脉冲计量学以及各个研究领域中极端时间尺度下的动力学研究开辟了新机遇。