Department of Condensed Matter Physics, J. Stefan Institute, SI-1000 Ljubljana, Slovenia.
Faculty of Mathematics and Physics, University of Ljubljana, SI-1000 Ljubljana, Slovenia.
Proc Natl Acad Sci U S A. 2021 Dec 7;118(49). doi: 10.1073/pnas.2110839118.
Liquid crystals (LCs) form an extremely rich range of self-assembled topological structures with artificially or naturally created topological defects. Some of the main applications of LCs are various optical and photonic devices, where compared to their solid-state counterparts, soft photonic systems are fundamentally different in terms of unique properties such as self-assembly, self-healing, large tunability, sensitivity to external stimuli, and biocompatibility. Here we show that complex tunable microlasers emitting structured light can be generated from self-assembled topological LC superstructures containing topological defects inserted into a thin Fabry-Pérot microcavity. The topology and geometry of the LC superstructure determine the structuring of the emitted light by providing complex three-dimensionally varying optical axis and order parameter singularities, also affecting the topology of the light polarization. The microlaser can be switched between modes by an electric field, and its wavelength can be tuned with temperature. The proposed soft matter microlaser approach opens directions in soft matter photonics research, where structured light with specifically tailored intensity and polarization fields could be designed and implemented.
液晶(LC)形成了极其丰富的自组装拓扑结构范围,具有人为或自然产生的拓扑缺陷。LC 的一些主要应用是各种光学和光子学器件,与它们的固态对应物相比,软光子学系统在自组装、自修复、大可调谐性、对外界刺激的敏感性和生物相容性等独特性质方面存在根本差异。在这里,我们展示了可以从包含拓扑缺陷的自组装拓扑 LC 超结构中产生复杂可调谐的发射结构光的微激光器,该超结构插入到薄的法布里-珀罗微腔中。LC 超结构的拓扑和几何形状通过提供复杂的三维变化的光轴和序参数奇点来确定发射光的结构,也会影响光偏振的拓扑结构。微激光器可以通过电场在模式之间切换,其波长可以随温度进行调谐。所提出的软物质微激光器方法为软物质光子学研究开辟了方向,在该研究中,可以设计和实现具有特定调制强度和偏振场的结构光。