Department of Mechanical Science and Engineering, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801, USA.
The Beckman Institute for Advanced Science and Technology, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801, USA.
Soft Matter. 2022 Jan 5;18(2):262-271. doi: 10.1039/d1sm01376a.
Drying of fine hair and fibers induces dramatic capillary-driven deformation, with important implications on natural phenomena and industrial processes. We recently observed peculiar self-assembly of hair bundles into various distinct patterns depending on the interplay between the bundle length and the liquid drain rate. Here, we propose a mechanism for this pattern selection, and derive and validate theoretical scaling laws for the polymorphic self-assembly of polygonal hair bundles. Experiments are performed by submerging the bundles into a liquid bath, then draining down the liquid. Depending on the interplay between the drain rates and the length of the fibers, we observe the bundles morphing into stars (having concave sides), polygons (having straight edges and rounded corners), or circles. The mechanism of self-assembly at the high drain regime is governed by two sequential stages. In the first stage of the high drain rate regime, the liquid covers the outside of the bundles, and drainage from inside the bundle does not play a role in the self-assembly due to the high viscous stress. The local pressure at the corners of the wet bundles compresses the fibers inward blunting the corners, and the internal lubrication facilitates fiber rearrangement. In the second stage, the liquid is slowly draining from within the fiber spacing, and the negative capillary pressure at the perimeter causes the fibers to tightly pack. In the slow drainage regime, the first stage is absent, and the fibers slowly aggregate without initial dynamic rearrangement. Understanding the mechanism of dynamic elastocapillarity offers insights for studying the complicated physics of wet granular drying.
细毛发和纤维的干燥会引起显著的毛细驱动变形,这对自然现象和工业过程都有重要影响。我们最近观察到,毛发束会根据束长和液体排出速率之间的相互作用,形成各种不同的独特自组装图案。在这里,我们提出了这种图案选择的机制,并推导出了用于多边形毛发束多态自组装的理论标度律,并进行了验证。实验是通过将束浸入液体浴中,然后排出液体来进行的。根据排出速率和纤维长度之间的相互作用,我们观察到束状结构会变形为星形(具有凹面)、多边形(具有直边和圆角)或圆形。在高排出率的自组装机制由两个连续阶段控制。在高排出率阶段的第一阶段,液体覆盖在束的外部,由于高粘性应力,内部的束排水对自组装没有作用。湿束角处的局部压力向内压缩纤维,使角变钝,内部润滑促进纤维重新排列。在第二阶段,液体从纤维间距内缓慢排出,周界处的负毛细压力导致纤维紧密堆积。在缓慢排出率下,第一阶段不存在,纤维在没有初始动态重新排列的情况下缓慢聚集。了解动态弹性毛细作用的机制为研究湿颗粒干燥的复杂物理提供了思路。