Valerio-Cuadros Marlon Ivan, Chaves Davi Araujo Dalbuquerque, Colauto Fabiano, Oliveira Ana Augusta Mendonça de, Andrade Antônio Marcos Helgueira de, Johansen Tom Henning, Ortiz Wilson Aires, Motta Maycon
Departamento de Física, Universidade Federal de São Carlos, São Carlos 13565-905, SP, Brazil.
Instituto Federal de Educação, Ciência e Tecnologia de São Paulo, Campus São Carlos, São Carlos 13565-905, SP, Brazil.
Materials (Basel). 2021 Nov 28;14(23):7274. doi: 10.3390/ma14237274.
Granularity is one of the main features restricting the maximum current which a superconductor can carry without losses, persisting as an important research topic when applications are concerned. To directly observe its effects on a typical thin superconducting specimen, we have modeled the simplest possible granular system by fabricating a single artificial weak-link in the center of a high-quality Nb film using the focused ion beam technique. Then, its microstructural, magnetic, and electric properties in both normal and superconducting states were studied. AC susceptibility, DC magnetization, and magneto-transport measurements reveal well-known granularity signatures and how they negatively affect superconductivity. Moreover, we also investigate the normal state electron scattering mechanisms in the Boltzmann theory framework. The results clearly demonstrate the effect of the milling technique, giving rise to an additional quadratic-in-temperature contribution to the usual cubic-in-temperature band scattering for the Nb film. Finally, by analyzing samples with varying density of incorporated defects, the emergence of the additional contribution is correlated to a decrease in their critical temperature, in agreement with recent theoretical results.
粒度是限制超导体在无损耗情况下所能承载的最大电流的主要特征之一,在涉及应用时,它一直是一个重要的研究课题。为了直接观察其对典型薄超导样品的影响,我们通过使用聚焦离子束技术在高质量铌薄膜中心制造单个人工弱连接,对最简单的可能的粒状系统进行了建模。然后,研究了其在正常和超导状态下的微观结构、磁性和电学性质。交流磁化率、直流磁化强度和磁输运测量揭示了众所周知的粒度特征以及它们如何对超导性产生负面影响。此外,我们还在玻尔兹曼理论框架内研究了正常态电子散射机制。结果清楚地证明了研磨技术的影响,导致铌薄膜在通常的与温度的三次方成比例的能带散射之外,出现了一个与温度的二次方成比例的额外贡献。最后,通过分析具有不同掺入缺陷密度的样品,额外贡献的出现与它们的临界温度降低相关,这与最近的理论结果一致。