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氧化锰改性生物炭:从水溶液中去除污染物的生产、特性及应用综述。

Manganese oxide-modified biochar: production, characterization and applications for the removal of pollutants from aqueous environments - a review.

机构信息

University of Wuppertal, School of Architecture and Civil Engineering, Institute of Foundation Engineering, Water- and Waste-Management, Laboratory of Soil- and Groundwater-Management, Pauluskirchstraße 7, 42285 Wuppertal, Germany; King Abdulaziz University, Faculty of Meteorology, Environment, and Arid Land Agriculture, Department of Arid Land Agriculture, 21589 Jeddah, Saudi Arabia; University of Kafrelsheikh, Faculty of Agriculture, Department of Soil and Water Sciences, 33516, Kafr El-Sheikh, Egypt.

Department of Environmental Sciences, COMSATS University Islamabad, Vehari Campus, Vehari, Pakistan.

出版信息

Bioresour Technol. 2022 Feb;346:126581. doi: 10.1016/j.biortech.2021.126581. Epub 2021 Dec 16.

Abstract

The development of manganese (Mn) oxides (MnOx) modified biochar (MnOBC) for the removal of pollutants from water has received significant attention. However, a comprehensive review focusing on the use of MnOBC for the removal of organic and inorganic pollutants from water is missing. Therefore, the preparation and characterization of MnOBC, and its capacity for the removal of inorganic (e.g., toxic elements) and organic (e.g., antibiotics and dyes) from water have been discussed in relation to feedstock properties, pyrolysis temperature, modification ratio, and environmental conditions here. The removal mechanisms of pollutants by MnOBC and the fate of the sorbed pollutants onto MnOBC have been reviewed. The impregnation of biochar with MnOx improved its surface morphology, functional group modification, and elemental composition, and thus increased its sorption capacity. This review establishes a comprehensive understanding of synthesizing and using MnOBC as an effective biosorbent for remediation of contaminated aqueous environments.

摘要

用于去除水中污染物的锰 (Mn) 氧化物 (MnOx) 改性生物炭 (MnOBC) 的开发受到了广泛关注。然而,目前缺少针对 MnOBC 用于去除水中有机和无机污染物的全面综述。因此,本文讨论了 MnOBC 的制备和表征及其去除水中无机(如有毒元素)和有机(如抗生素和染料)污染物的能力,重点讨论了原料特性、热解温度、改性比和环境条件的影响。还综述了 MnOBC 去除污染物的机制以及被吸附污染物在 MnOBC 上的归宿。MnOx 浸渍生物炭可改善其表面形态、官能团修饰和元素组成,从而提高其吸附能力。本综述建立了对合成和使用 MnOBC 作为有效生物吸附剂修复受污染水环境的全面理解。

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