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铒铁氧体单晶中自旋翻转的低场控制与连续磁转变

Low field control of spin switching and continuous magnetic transition in an ErFeO single crystal.

作者信息

Ma Xiaoxuan, Fan Wencheng, Zhao Gang, Chen Haiyang, Wang Chuankun, Kang Baojuan, Feng Zhenjie, Ge Jun-Yi, Ren Wei, Cao Shixun

机构信息

Department of Physics, Materials Genome Institute, International Center for Quantum and Molecular Structures, Shanghai University, Shanghai 200444, China.

Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai 200444, China.

出版信息

Phys Chem Chem Phys. 2022 Jan 4;24(2):735-742. doi: 10.1039/d1cp04668c.

Abstract

The magnetic behavior of a rare-earth orthoferrite ErFeO single crystal can be controlled by low magnetic fields from a few to hundreds of Oe. Here we investigated a high-quality ErFeO single crystal in the temperature range of 5-120 K, with two types of spin switching in the field-cooled-cooling (FCC) and field-cooled-warming (FCW) processes below the temperature of the spin reorientation (SR) transition from Γ to Γ at 98-88 K. The magnitude of the applied magnetic fields can regulate two types of spin switching along the -axis of the ErFeO single crystal but does not affect the type and temperature range of the SR transition. An interesting "multi-step" type-II spin switching is observed in FCW under low magnetic fields ( < 18 Oe) just below the SR transition temperature, which is associated with the interaction and the change of magnetic configurations from rare-earth and iron magnetic sublattices. When the magnetic field is lower than 15 Oe, the type-II spin switching in the FCW process gradually changes to a continuous magnetic transition along the -axis of the ErFeO single crystal. As the magnetic field is reduced to less than 17 Oe, the type-I spin switching in the FCW process also transforms into a continuous magnetic transition. Understanding the magnetic reversal effects will help us explore the potential applications of these magnetic materials for future information devices.

摘要

稀土正铁氧体ErFeO单晶的磁行为可由几到几百奥斯特的低磁场控制。在此,我们研究了一种高质量的ErFeO单晶,其温度范围为5 - 120 K,在98 - 88 K从Γ到Γ的自旋重取向(SR)转变温度以下的场冷冷却(FCC)和场冷热(FCW)过程中存在两种类型的自旋切换。施加磁场的大小可以调节沿ErFeO单晶z轴的两种类型的自旋切换,但不影响SR转变的类型和温度范围。在略低于SR转变温度的低磁场(< 18 Oe)下的FCW过程中观察到一种有趣的“多步”II型自旋切换,这与稀土和铁磁性亚晶格的相互作用以及磁构型的变化有关。当磁场低于15 Oe时,FCW过程中的II型自旋切换逐渐变为沿ErFeO单晶z轴的连续磁转变。随着磁场降低到小于17 Oe,FCW过程中的I型自旋切换也转变为连续磁转变。理解磁反转效应将有助于我们探索这些磁性材料在未来信息设备中的潜在应用。

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