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基于液相色谱-质谱联用的代谢组学区分不同山谷的智利赤霞珠优质葡萄酒和标准葡萄酒。

LC-MS-Based Metabolomics Discriminates Premium from Standard Chilean cv. Cabernet Sauvignon Wines from Different Valleys.

作者信息

Sáez Vania, Schober Doreen, González Álvaro, Arapitsas Panagiotis

机构信息

Department of Food Quality and Nutrition, Research and Innovation Centre, Fondazione Edmund Mach, Via Edmund Mach 1, 38010 San Michele All'Adige, Italy.

Center for Research and Innovation, Viña Concha y Toro, Ruta K-650 Km 10, Pencahue 3550000, Chile.

出版信息

Metabolites. 2021 Nov 30;11(12):829. doi: 10.3390/metabo11120829.

DOI:10.3390/metabo11120829
PMID:34940587
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC8707972/
Abstract

Cabernet Sauvignon grapes in Chile, mainly grown between the 30° S and 36° S, account for more than 30% of Chilean wine production, and yield wines with different characteristics which influence their quality. The aim of this study was to apply a liquid chromatography-mass spectrometry (LC-MS)-based metabolomic protocol to investigate the quality differentiation in a sample set of monovarietal wines from eight valleys covering 679 km of the north-south extension. All samples were produced using a standardized red winemaking process and classified according to a company categorization in two major groups: premium and standard, and each group in two subcategories. The results pointed out that N-containing metabolites (mainly small peptides) are promising biomarkers for quality differentiation. Moreover, the premium wines were characterized by higher amounts of anthocyanins and other glycosylated and acetylated flavonoids, as well as phenolic acids; standard quality wines, on the other hand, presented stilbenoids and sulfonated catabolites of tryptophan and flavanols.

摘要

智利的赤霞珠葡萄主要种植在南纬30°至36°之间，占智利葡萄酒产量的30%以上，所产葡萄酒具有不同特性，影响其品质。本研究旨在应用基于液相色谱 - 质谱联用（LC - MS）的代谢组学方法，对来自八个山谷、南北延伸679公里的单一品种葡萄酒样本集的品质差异进行研究。所有样本均采用标准化的红葡萄酒酿造工艺生产，并根据公司分类分为两个主要类别：优质和标准，每个类别再分为两个子类别。结果表明，含氮代谢物（主要是小肽）是品质差异的潜在生物标志物。此外，优质葡萄酒的特点是花青素和其他糖基化及乙酰化黄酮类化合物以及酚酸含量较高；另一方面，标准品质葡萄酒含有芪类化合物以及色氨酸和黄烷醇的磺化分解产物。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/b2060722e1cb/metabolites-11-00829-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/dc59a81a505c/metabolites-11-00829-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/3ad3f4ed9e47/metabolites-11-00829-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/19e3ec98a012/metabolites-11-00829-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/0b30c17d0fee/metabolites-11-00829-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/950ee8fa6f68/metabolites-11-00829-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/5cb1f87b8fe1/metabolites-11-00829-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/b2060722e1cb/metabolites-11-00829-g007.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/dc59a81a505c/metabolites-11-00829-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/3ad3f4ed9e47/metabolites-11-00829-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/19e3ec98a012/metabolites-11-00829-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/0b30c17d0fee/metabolites-11-00829-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/950ee8fa6f68/metabolites-11-00829-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/5cb1f87b8fe1/metabolites-11-00829-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9651/8707972/b2060722e1cb/metabolites-11-00829-g007.jpg

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