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[昭通市周边扬尘中重金属污染特征及健康风险]

[Pollution Characteristics and Health Risk of Heavy Metals in Fugitive Dust Around Zhaotong City].

作者信息

Pang Xiao-Chen, Han Xin-Yu, Shi Jian-Wu, Bao Yu-Zhai, Ning Ping, Zhang Chao-Neng, Xiang Feng

机构信息

Faculty of Environmental Science and Engineering, Kunming University of Science and Technology, Kunming 650500, China.

Faculty of Civil Engineering and Architectural, Kunming University of Science and Technology, Kunming 650500, China.

出版信息

Huan Jing Ke Xue. 2022 Jan 8;43(1):180-188. doi: 10.13227/j.hjkx.202106018.

Abstract

In order to explore the pollution characteristics and health risks of heavy metals in fugitive dust around the urban areas of Zhaotong City, road dust and soil dust samples were collected in the Zhaoyang District of Zhaotong City in May 2019. The dust samples were suspended using a particle resuspension system to obtain PM (particulate matter with an aerodynamic diameter less than or equal to 2.5 μm). The concentrations of Ca, Al, Fe, Mg, Ti, V, Cr, Mn, Co, Ni, Cu, Zn, As, Cd, and Pb in PM were quantified by ICP-MS and ICP-OES. By analyzing 10 types of heavy metals in PM, the results showed that the average concentration of Mn was the highest in the soil fugitive dust, followed by Cr, Ni, Zn, Cu, Co, Pb, V, As, and Cd. The average concentration of Zn in the road fugitive dust was the highest, followed by Mn, Cu, Cr, Pb, Ni, As, Co, V, and Cd. The enrichment factor (EF) indicated that Cd was strongly enriched in the two types of fugitive dust. The EFs of Cu, Zn, and Pb in road fugitive dust showed a moderate enrichment, and they were higher than those in soil fugitive dust. Correlation and principal component analysis showed that heavy metals in the two types of fugitive dust were affected by coal burning sources. At the same time, heavy metals in soil fugitive dust were affected by agricultural activity sources, and heavy metals in road fugitive dust were affected by traffic sources. The results of the health risk assessment indicated that the carcinogenic risks of Cr, Co, Ni, As, and Cd in soil fugitive dust were higher than those in road fugitive dust. The non-carcinogenic risks of heavy metals in the two types of fugitive dust for children were higher than those for adults, and the non-carcinogenic risks of Cu, Zn, and Pb in road fugitive dust were higher than those in soil fugitive dust.

摘要

为探究昭通市城区周边扬尘中重金属的污染特征及健康风险,于2019年5月在昭通市昭阳区采集了道路扬尘和土壤扬尘样本。利用颗粒物再悬浮系统将扬尘样本悬浮,以获取PM(空气动力学直径小于或等于2.5μm的颗粒物)。采用电感耦合等离子体质谱仪(ICP-MS)和电感耦合等离子体发射光谱仪(ICP-OES)对PM中Ca、Al、Fe、Mg、Ti、V、Cr、Mn、Co、Ni、Cu、Zn、As、Cd和Pb的浓度进行定量分析。通过分析PM中的10种重金属,结果表明,土壤扬尘中Mn的平均浓度最高,其次是Cr、Ni、Zn、Cu、Co、Pb、V、As和Cd。道路扬尘中Zn的平均浓度最高,其次是Mn、Cu、Cr、Pb、Ni、As、Co、V和Cd。富集因子(EF)表明,Cd在两种扬尘中均有强烈富集。道路扬尘中Cu、Zn和Pb的EF显示出中等程度富集,且高于土壤扬尘中的富集程度。相关性分析和主成分分析表明,两种扬尘中的重金属受燃煤源影响。同时,土壤扬尘中的重金属受农业活动源影响,道路扬尘中的重金属受交通源影响。健康风险评估结果表明,土壤扬尘中Cr、Co、Ni、As和Cd的致癌风险高于道路扬尘。两种扬尘中重金属对儿童的非致癌风险高于成人,且道路扬尘中Cu、Zn和Pb的非致癌风险高于土壤扬尘。

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