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[太原市采暖季城乡室内灰尘重金属污染特征及生态风险评价]

[Characteristics of Heavy Metal Pollution and Ecological Risk Evaluation of Indoor Dust from Urban and Rural Areas in Taiyuan City During the Heating Season].

作者信息

Huang Hao, Xu Zi-Qi, Yan Jun-Xia, Zhao Xiu-Ge, Wang Dan-Lu

机构信息

Institute of Loess Plateau, Shanxi University, Taiyuan 030006, China.

Department of Environmental Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, China.

出版信息

Huan Jing Ke Xue. 2021 May 8;42(5):2143-2152. doi: 10.13227/j.hjkx.202008045.

Abstract

The presence of heavy metals in indoor dust is a world-wide concern owing to its negative impact on humans. In this study, we collected indoor dust samples from urban and rural residential areas during the heating season in Taiyuan City. We then identified the concentrations of 11 heavy metals (Cd, Co, Cr, Pb, Mn, Ni, Cu, Zn, V, As, and Hg) using inductively coupled plasma-mass spectrometry. Based on the concentrations, we categorized the pollution levels of indoor dust using the geo-accumulation index and the pollution load index. We further identified the sources of heavy metals using the enrichment factor and principal component analysis. Finally, we evaluated the potential ecological risks of heavy metals via the potential ecological index. The results illustrated that ① with the exception of Co, Mn, and V, the mean concentrations of Cd, Cr, Cu, Ni, Pb, As, Zn, and Hg in indoor dust were higher than the soil background values of Shanxi Province. There was a significant difference (<0.05) in the concentrations of Co, Cr, Cu, Mn, Ni, and Hg between the urban and rural areas. ② Overall, the pollution degree of heavy metals in indoor dust was identified as moderate in the urban area of Taiyuan City, but slight in the rural area. The indoor dust sample in the urban area was not contaminated by Co, Mn, and V. However, it was slightly polluted by As, Ni, and Hg. In addition, it was close to moderately polluted by Cd, Cr, Cu, Pb, and Zn. In the rural area, the pollution degrees of all the metals, except for Hg and V, in indoor dust were lower than those in the urban area. ③ The As, Cd, Cu, Pb, Zn, and Hg in indoor dust for both urban and rural areas might have mainly originated from anthropogenic sources. The pollution sources were mainly transportation and industry in the urban area and coal combustion and indoor smoking in the rural area. The Co, Cr, Mn, Ni, and V in indoor dust in Taiyuan City might have mainly originated from natural sources. ④ The ecological risk of heavy metal pollution in indoor dust for both the urban and rural areas of Taiyuan City was relatively high, with integrated ecological risk indexes of 359.43 and 471.02 in the urban and rural areas, respectively. In addition, Cd and Hg were the largest contributors.

摘要

由于室内灰尘中的重金属对人类有负面影响,其在全球范围内受到关注。在本研究中,我们在太原市供暖季期间从城市和农村居民区采集了室内灰尘样本。然后,我们使用电感耦合等离子体质谱法测定了11种重金属(镉、钴、铬、铅、锰、镍、铜、锌、钒、砷和汞)的浓度。基于这些浓度,我们用地积累指数和污染负荷指数对室内灰尘的污染水平进行了分类。我们还使用富集因子和主成分分析确定了重金属的来源。最后,我们通过潜在生态指数评估了重金属的潜在生态风险。结果表明:①除钴、锰和钒外,室内灰尘中镉、铬、铜、镍、铅、砷、锌和汞的平均浓度高于山西省土壤背景值。城市和农村地区钴、铬、铜、锰、镍和汞的浓度存在显著差异(<0.05)。②总体而言,太原市城区室内灰尘中重金属污染程度为中度,农村地区为轻度。城区室内灰尘样本未受钴、锰和钒污染。然而,它受到砷、镍和汞的轻度污染。此外,它受到镉、铬、铜、铅和锌的接近中度污染。在农村地区,室内灰尘中除汞和钒外的所有金属污染程度均低于城区。③城区和农村地区室内灰尘中的砷、镉、铜、铅、锌和汞可能主要来自人为源。城区污染源主要是交通和工业,农村地区是煤炭燃烧和室内吸烟。太原市室内灰尘中的钴、铬、锰、镍和钒可能主要来自自然源。④太原市城区和农村地区室内灰尘中重金属污染的生态风险相对较高,城区和农村地区的综合生态风险指数分别为359.43和471.02。此外,镉和汞是最大的贡献者。

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