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CdZnTeSe在偏压下的低温退火

Low-Temperature Annealing of CdZnTeSe under Bias.

作者信息

Rejhon Martin, Dedic Vaclav, Grill Roman, Franc Jan, Roy Utpal N, James Ralph B

机构信息

Faculty of Mathematics and Physics, Charles University, Ke Karlovu 3, 12116 Prague, Czech Republic.

Tandon School of Engineering, New York University, Brooklyn, NY 11201, USA.

出版信息

Sensors (Basel). 2021 Dec 28;22(1):171. doi: 10.3390/s22010171.

DOI:10.3390/s22010171
PMID:35009714
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC8747470/
Abstract

We performed a gradual low-temperature annealing up to 360 K on a CdZnTeSe radiation detector equipped with gold and indium electrodes under bias at both polarities. We observed significant changes in the detector's resistance and space-charge accumulation. This could potentially lead to the control and improvement of the electronic properties of the detector because the changes are accompanied with the reduction in the bulk dark current and surface leakage current. In this article, we present the results of a detailed study of the internal electric field and conductivity changes in CdZnTeSe detector for various annealing steps under bias taking into account different polarities during annealing and subsequent characterization. We observed that low-temperature annealing results in an increase in the barrier height at the contacts that, in general, reduces the dark current and decreases the positive space charge present in the sample compared to the pre-annealed condition.

摘要

我们在一个配备金和铟电极的CdZnTeSe辐射探测器上,在两种极性的偏压下进行了逐步升温至360K的低温退火。我们观察到探测器电阻和空间电荷积累有显著变化。这可能潜在地导致探测器电子性能的控制和改善,因为这些变化伴随着体暗电流和表面漏电流的降低。在本文中,我们展示了在考虑退火过程中的不同极性以及后续表征的情况下,对处于偏压下的CdZnTeSe探测器在不同退火步骤下内部电场和电导率变化的详细研究结果。我们观察到低温退火导致接触处势垒高度增加,总体而言,与退火前的状态相比,这降低了暗电流并减少了样品中存在的正空间电荷。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/f67c60ea1de4/sensors-22-00171-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/632c5333ce3b/sensors-22-00171-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/563032b2b7ad/sensors-22-00171-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/dd9394691783/sensors-22-00171-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/626bdb87c669/sensors-22-00171-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/a299e917b731/sensors-22-00171-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/f67c60ea1de4/sensors-22-00171-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/632c5333ce3b/sensors-22-00171-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/563032b2b7ad/sensors-22-00171-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/dd9394691783/sensors-22-00171-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/626bdb87c669/sensors-22-00171-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/a299e917b731/sensors-22-00171-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4e3a/8747470/f67c60ea1de4/sensors-22-00171-g006.jpg

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本文引用的文献

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Impact of selenium addition to the cadmium-zinc-telluride matrix for producing high energy resolution X-and gamma-ray detectors.向碲化镉锌基体中添加硒对生产高能量分辨率X射线和伽马射线探测器的影响。
Sci Rep. 2021 May 14;11(1):10338. doi: 10.1038/s41598-021-89795-z.
2
Evaluation of CdZnTeSe as a high-quality gamma-ray spectroscopic material with better compositional homogeneity and reduced defects.评估碲锌镉硒作为一种具有更好成分均匀性和减少缺陷的高质量伽马射线光谱材料。
Sci Rep. 2019 May 13;9(1):7303. doi: 10.1038/s41598-019-43778-3.
3
Role of selenium addition to CdZnTe matrix for room-temperature radiation detector applications.
向CdZnTe基体中添加硒在室温辐射探测器应用中的作用。
Sci Rep. 2019 Feb 7;9(1):1620. doi: 10.1038/s41598-018-38188-w.
4
Exploring the validity and limitations of the Mott-Gurney law for charge-carrier mobility determination of semiconducting thin-films.探索莫特-格尼定律在确定半导体薄膜载流子迁移率方面的有效性和局限性。
J Phys Condens Matter. 2018 Mar 14;30(10):105901. doi: 10.1088/1361-648X/aaabad.