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具有高优值的低维纳米结构辅助远程表面等离子体共振传感器

Low Dimensional Nanostructure-Assisted Long-Range Surface Plasmon Resonance Sensors With High Figure of Merit.

作者信息

Wang Qi, Cong Xue-Wei, Cheng Zhan, Zhao Wan-Ming, Wang Lei, Yin Xiang-Yu, Jiang Ju-Xin, Ren Zi-Han, Yan Xin, Zhu Ai-Song, Qiu Feng-Mei, Chen Bin-Hai, Zhang Ke-Ke

出版信息

IEEE Trans Nanobioscience. 2023 Jan;22(1):45-51. doi: 10.1109/TNB.2022.3149513. Epub 2022 Dec 29.

Abstract

Long-range surface plasmon resonance (LRSPR) sensors have been extensively studied by virtue of their extremely narrow full width at half maxima (FWHM) characteristics, but their low sensitivity remains an important factor limiting the figure of merit (FOM), making the sensors have difficulties in detecting small refractive index changes accurately. To address this problem, this paper proposes and demonstrates a low dimensional nanostructure (Au nanospheres, WS2) assisted LRSPR sensor to achieve an effective enhancement of the sensor interfaced electric field and thus improve the sensitivity. The performance parameters of the two sensors are compared with the LRSPR sensor by finite element method analysis, and the results showed that the assistance of the low dimensional nanostructure has a positive effect on the sensor. The first refractive index sensing experiment of the WS2-assisted LRSPR sensor was realized with a 25.47% increase in sensitivity and a 7.13% increase in FOM simultaneously, and the Au nanospheres-assisted LRSPR sensor with a 29.23% increase in sensitivity and a 15.95% increase in FOM simultaneously. The introduction of low dimensional nanostructures provides a flexible and effective means of sensitization for LRSPR sensors, making the plasmon resonance sensors combine high sensitivity, narrow FWHM and high FOM, which have promising applications in biochemical sensing.

摘要

长程表面等离子体共振(LRSPR)传感器因其半高宽(FWHM)极窄的特性而受到广泛研究,但其低灵敏度仍是限制品质因数(FOM)的重要因素,导致传感器难以准确检测微小的折射率变化。为解决这一问题,本文提出并展示了一种低维纳米结构(金纳米球、二硫化钨)辅助的LRSPR传感器,以有效增强传感器界面电场,从而提高灵敏度。通过有限元方法分析,将这两种传感器的性能参数与LRSPR传感器进行比较,结果表明低维纳米结构的辅助对传感器有积极影响。实现了二硫化钨辅助的LRSPR传感器的首次折射率传感实验,灵敏度同时提高了25.47%,FOM提高了7.13%,金纳米球辅助的LRSPR传感器灵敏度同时提高了29.23%,FOM提高了15.95%。低维纳米结构的引入为LRSPR传感器提供了一种灵活有效的敏化手段,使等离子体共振传感器兼具高灵敏度、窄FWHM和高FOM,在生化传感方面具有广阔的应用前景。

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