Key Laboratory of Advanced Technologies of Materials (Ministry of Education), School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu 610031, China.
Key Laboratory of Advanced Technologies of Materials (Ministry of Education), School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu 610031, China; Institute of Frontier Science and Technology, Southwest Jiaotong University, Chengdu 610031, PR China.
J Colloid Interface Sci. 2022 Jun;615:215-226. doi: 10.1016/j.jcis.2022.01.117. Epub 2022 Jan 20.
Conductive hydrogel has been considered as a promising material for wearable sensors, constructing a flexible conductive hydrogel sensor with super stretchability, adhesion, and sensing stability is essential, but still challenging. Herein, A super-stretchable, adhesive, and conductive nanocomposite hydrogel was successfully constructed by a facile and one-pot process in conjunction with ball milling and blending. The resulting hydrogel exhibited super-stretchable ability (2795%), excellent tensile stress (128.6 kPa), good fatigue resistance, and self-recovery ability due to multiple cross-linked network structures, including physical hybrid networks (hydrogen bonds and ionic coordination bonds) and flexible polyacrylamide networks. Moreover, the nanocomposite hydrogel showed outstanding conductivity stability, fast response, durability, and repeatability. And it displayed excellent adhesion on various materials. Strain sensors based on hydrogels showed high sensitivity, stability, and action recognition ability. In summary, this work provides a simple strategy for preparing conductive hydrogel sensors with high stretchability, adhesion, and stability, and has potential application prospects in the field of wearable sensors for human body motion detection.
导电水凝胶已被认为是一种有前途的可穿戴传感器材料,构建具有超拉伸性、附着力和传感稳定性的柔性导电水凝胶传感器至关重要,但仍具有挑战性。在此,通过简单的一锅法结合球磨和共混,成功构建了一种超拉伸、高附着力和导电的纳米复合水凝胶。由于存在多种交联网络结构,包括物理混合网络(氢键和离子配位键)和柔性聚丙烯酰胺网络,所得水凝胶表现出超拉伸能力(2795%)、优异的拉伸应力(128.6kPa)、良好的耐疲劳性和自恢复能力。此外,纳米复合水凝胶表现出出色的电导率稳定性、快速响应、耐久性和可重复性。并且它在各种材料上表现出优异的附着力。基于水凝胶的应变传感器具有高灵敏度、稳定性和动作识别能力。总之,这项工作为制备具有高拉伸性、附着力和稳定性的导电水凝胶传感器提供了一种简单的策略,在人体运动检测的可穿戴传感器领域具有潜在的应用前景。
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