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奥帕林斯黏土层内断层岩的物理特性

Physical characterization of fault rocks within the Opalinus Clay formation.

作者信息

Orellana Luis Felipe, Nussbaum Christophe, Grafulha Luiz, Henry Pierre, Violay Marie

机构信息

Laboratory of Experimental Rock Mechanics, IIC-ENAC, École Polytechnique Fédérale de Lausanne, Lausanne, Switzerland.

Now Department of Mining Engineering, FCFM - Universidad de Chile, Santiago, Chile.

出版信息

Sci Rep. 2022 Mar 14;12(1):4389. doi: 10.1038/s41598-022-08236-7.

DOI:10.1038/s41598-022-08236-7
PMID:35288596
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC8921326/
Abstract

Near-surface disposal of radioactive waste in shales is a promising option to safeguard the population and environment. However, natural faults intersecting these geological formations can potentially affect the long-term isolation of the repositories. This paper characterizes the physical properties and mineralogy of the internal fault core structure intersecting the Opalinus Clay formation, a host rock under investigation for nuclear waste storage at the Mont Terri Laboratory (Switzerland). We have performed porosity, density, microstructural and mineralogical measurements in different sections of the fault, including intact clays, scaly clays and fault gouge. Mercury intrusion porosimetry analysis reveal a gouge that has a pore network dominated by nanopores of less than 10 nm, yet a high-porosity (21%) and low grain density (2.62 g/cm) when compared to the intact rock (14.2%, and 2.69 g/cm). Thus, a more permeable internal fault core structure with respect to the surrounding rock is deduced. Further, we describe the OPA fault gouge as a discrete fault structure having the potential to act as a preferential, yet narrow, and localized channel for fluid-flow if compared to the surrounding rock. Since the fault gouge is limited to a millimetres-thick structure, we expect the barrier property of the geological formation is almost not affected.

摘要

在页岩中进行放射性废物的近地表处置是保障公众和环境安全的一个有前景的选择。然而,与这些地质构造相交的天然断层可能会对储存库的长期隔离产生潜在影响。本文描述了与奥帕林努斯粘土层相交的内部断层核心结构的物理性质和矿物学特征,奥帕林努斯粘土是瑞士蒙特特里实验室正在研究的用于核废料储存的主岩。我们对断层的不同部分进行了孔隙度、密度、微观结构和矿物学测量,包括完整粘土、鳞片粘土和断层泥。压汞孔隙度分析表明,断层泥具有以小于10纳米的纳米孔为主的孔隙网络,但与完整岩石(14.2%和2.69克/立方厘米)相比,其孔隙度较高(21%)且颗粒密度较低(2.62克/立方厘米)。因此,可以推断出内部断层核心结构相对于周围岩石具有更高的渗透性。此外,与周围岩石相比,我们将OPA断层泥描述为一种离散的断层结构,它有可能作为流体流动的优先通道,尽管该通道狭窄且局部化。由于断层泥仅限于毫米级厚度的结构,我们预计地质构造的阻隔性能几乎不会受到影响。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/bc0e67c8abad/41598_2022_8236_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/eb7ac7c04c4c/41598_2022_8236_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/4614f590d02f/41598_2022_8236_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/a5cf853ae7f5/41598_2022_8236_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/bc0e67c8abad/41598_2022_8236_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/eb7ac7c04c4c/41598_2022_8236_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/4614f590d02f/41598_2022_8236_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/a5cf853ae7f5/41598_2022_8236_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/ad76/8921326/bc0e67c8abad/41598_2022_8236_Fig4_HTML.jpg

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本文引用的文献

1
The Nanoscale Basis of CO2 Trapping for Geologic Storage.二氧化碳地质封存的纳米基础。
Environ Sci Technol. 2015 Sep 1;49(17):10265-84. doi: 10.1021/acs.est.5b03003. Epub 2015 Aug 20.
2
Anisotropic diffusion in layered argillaceous rocks: a case study with Opalinus Clay.层状泥质岩中的各向异性扩散:以蛋白石黏土为例的研究
Environ Sci Technol. 2004 Nov 1;38(21):5721-8. doi: 10.1021/es049937g.
3
Mercury Intrusion Porosimetry and Image Analysis of Cement-Based Materials.水泥基材料的压汞孔隙率测定法及图像分析
J Colloid Interface Sci. 1999 Mar 1;211(1):39-44. doi: 10.1006/jcis.1998.5986.