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用氪离子束轰击的硅表面上的纳米级图案形成:实验与模拟

Nanoscale pattern formation on silicon surfaces bombarded with a krypton ion beam: experiments and simulations.

作者信息

Seo J, Pearson D A, Bradley R M, Kim J-S

机构信息

Institute of Advanced Materials and Systems, Sook-Myung Women's University, Seoul, 04310, Republic of Korea.

Division of Science and Engineering, Pennsylvania State University, Abington, Abington, PA 19001, United States of America.

出版信息

J Phys Condens Matter. 2022 Apr 27;34(26). doi: 10.1088/1361-648X/ac64df.

DOI:10.1088/1361-648X/ac64df
PMID:35385840
Abstract

The nanoscale patterns produced by bombardment of the (100) surface of silicon with a 2 keV Kr ion beam are investigated both experimentally and theoretically. In our experiments, we find that the patterns observed at high ion fluences depend sensitively on the angle of incidence Θ. For Θ values between 74° and 85°, we observe five decidedly different kinds of morphologies, including triangular nanostructures traversed by parallel-mode ripples, long parallel ridges decorated by short-wavelength ripples, and a remarkable mesh-like morphology. In contrast, only parallel-mode ripples are present for low ion fluences except for Θ = 85°. Our simulations show that triangular nanostructures that closely resemble those in our experiments emerge if a linearly dispersive term and a conserved Kuramoto-Sivashinsky nonlinearity are appended to the usual equation of motion. We find ridges traversed by ripples, on the other hand, in simulations of the Harrison-Pearson-Bradley equation (Harrison2017E032804). For Θ = 85°, the solid surface is apparently stable and simulations of an anisotropic Edwards-Wilkinson equation yield surfaces similar to those seen in our experiments. Explaining the other two kinds of patterns we find in our experiments remains a challenge for future theoretical work.

摘要

我们通过实验和理论研究了用2keV的Kr离子束轰击硅(100)表面所产生的纳米尺度图案。在我们的实验中,我们发现高离子注量下观察到的图案对入射角Θ敏感依赖。对于74°至85°之间的Θ值,我们观察到五种截然不同的形态,包括由平行模式波纹穿过的三角形纳米结构、由短波长波纹装饰的长平行脊以及一种显著的网状形态。相比之下,除了Θ = 85°外,低离子注量下仅存在平行模式波纹。我们的模拟表明,如果在通常的运动方程中附加一个线性色散项和一个守恒的Kuramoto-Sivashinsky非线性项,就会出现与我们实验中非常相似的三角形纳米结构。另一方面,在Harrison-Pearson-Bradley方程(Harrison2017E032804)的模拟中,我们发现了由波纹穿过的脊。对于Θ = 85°,固体表面显然是稳定的,并且各向异性Edwards-Wilkinson方程的模拟产生的表面与我们实验中看到的表面相似。解释我们在实验中发现的其他两种图案仍然是未来理论工作的一个挑战。

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