Guo Jiawen, Liu Huimin, Li Dezheng, Wang Jian, Djitcheu Xavier, He Dehua, Zhang Qijian
School of Chemical and Environmental Engineering, Liaoning University of Technology Jinzhou 121001 P. R. China
Innovative Catalysis Program, Key Lab of Organic Optoelectronics & Molecular Engineering of Ministry of Education, Department of Chemistry, Tsinghua University Beijing 100084 China.
RSC Adv. 2022 Mar 24;12(15):9373-9394. doi: 10.1039/d2ra00657j. eCollection 2022 Mar 21.
Single atom catalysis is a prosperous and rapidly growing research field, owing to the remarkable advantages of single atom catalysts (SACs), such as maximized atom utilization efficiency, tailorable catalytic activities as well as supremely high catalytic selectivity. Synthesis approaches play crucial roles in determining the properties and performance of SACs. Over the past few years, versatile methods have been adopted to synthesize SACs. Herein, we give a thorough and up-to-date review on the progress of approaches for the synthesis of SACs, outline the general principles and list the advantages and disadvantages of each synthesis approach, with the aim to give the readers a clear picture and inspire more studies to exploit novel approaches to synthesize SACs effectively.
单原子催化是一个蓬勃发展且快速增长的研究领域,这得益于单原子催化剂(SACs)具有的显著优势,例如最大化的原子利用效率、可定制的催化活性以及极高的催化选择性。合成方法在决定SACs的性质和性能方面起着关键作用。在过去几年中,人们采用了多种方法来合成SACs。在此,我们对SACs合成方法的进展进行全面且最新的综述,概述一般原则,并列出每种合成方法的优缺点,旨在让读者有清晰的了解,并激发更多研究以开发有效合成SACs的新方法。