Grbić Mihael S, O'Farrell Eoin C T, Matsumoto Yosuke, Kuga Kentaro, Brando Manuel, Küchler Robert, Nevidomskyy Andriy H, Yoshida Makoto, Sakakibara Toshiro, Kono Yohei, Shimura Yasuyuki, Sutherland Michael L, Takigawa Masashi, Nakatsuji Satoru
Institute for Solid State Physics (ISSP), University of Tokyo, Kashiwa, 277-8581, Japan.
Department of Physics, Faculty of Science, University of Zagreb, Bijenička 32, Zagreb, HR 10000, Croatia.
Nat Commun. 2022 Apr 19;13(1):2141. doi: 10.1038/s41467-022-29757-9.
Intermetallic compounds containing f-electron elements have been prototypical materials for investigating strong electron correlations and quantum criticality (QC). Their heavy fermion ground state evoked by the magnetic f-electrons is susceptible to the onset of quantum phases, such as magnetism or superconductivity, due to the enhanced effective mass (m) and a corresponding decrease of the Fermi temperature. However, the presence of f-electron valence fluctuations to a non-magnetic state is regarded an anathema to QC, as it usually generates a paramagnetic Fermi-liquid state with quasiparticles of moderate m. Such systems are typically isotropic, with a characteristic energy scale T of the order of hundreds of kelvins that require large magnetic fields or pressures to promote a valence or magnetic instability. Here we show the discovery of a quantum critical behaviour and a Lifshitz transition under low magnetic field in an intermediate valence compound α-YbAlB. The QC origin is attributed to the anisotropic hybridization between the conduction and localized f-electrons. These findings suggest a new route to bypass the large valence energy scale in developing the QC.
含f电子元素的金属间化合物一直是研究强电子关联和量子临界性(QC)的典型材料。由磁性f电子引起的重费米子基态易受量子相的影响,如磁性或超导性,这是由于有效质量(m)增加以及费米温度相应降低所致。然而,f电子价态向非磁性状态的涨落被认为是QC的克星,因为它通常会产生具有中等m的准粒子的顺磁费米液体状态。此类系统通常是各向同性的,具有数百开尔文量级的特征能量尺度T,需要强磁场或高压才能引发价态或磁性不稳定性。在此,我们展示了在中间价化合物α-YbAlB中低磁场下量子临界行为和里夫希茨转变的发现。量子临界起源归因于传导电子与局域f电子之间的各向异性杂化。这些发现为在发展量子临界性过程中绕过巨大的价态能量尺度提供了一条新途径。