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利用注入氪原子的同步加速器X射线荧光对炭黑生成的甲烷/空气火焰进行原位温度测量。

In situ temperature measurements in sooting methane/air flames using synchrotron x-ray fluorescence of seeded krypton atoms.

作者信息

Montgomery Matthew J, Kwon Hyunguk, Kastengren Alan L, Pfefferle Lisa D, Sikes Travis, Tranter Robert S, Xuan Yuan, McEnally Charles S

机构信息

Department of Chemical and Environmental Engineering, Yale University, New Haven, CT, USA.

Department of Chemical Engineering, Pennsylvania State University, University Park, PA, USA.

出版信息

Sci Adv. 2022 Apr 29;8(17):eabm7947. doi: 10.1126/sciadv.abm7947.

DOI:10.1126/sciadv.abm7947
PMID:35486725
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9054011/
Abstract

Synchrotron x-ray fluorescence has been used to measure temperatures in optically dense gases where traditional methods would fail. These data provide a benchmark for stringent tests of computational fluid dynamics models for complex systems where physical and chemical processes are intimately linked. The experiments measured krypton number densities in a sooting, atmospheric pressure, nonpremixed coflow flame that is widely used in combustion research. The experiments not only form targets for the models, but the simulations also identify potential sources of uncertainties in the measurements, allowing for future improvements.

摘要

同步辐射X射线荧光已被用于测量传统方法无法适用的光密气体中的温度。这些数据为对物理和化学过程紧密相连的复杂系统的计算流体动力学模型进行严格测试提供了基准。实验测量了一种广泛用于燃烧研究的、有烟灰生成的常压非预混并流火焰中的氪数密度。这些实验不仅为模型提供了目标,而且模拟还识别出测量中潜在的不确定来源,以便未来改进。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/569f26183f9c/sciadv.abm7947-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/b61104d60ae6/sciadv.abm7947-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/e69a386a5f8b/sciadv.abm7947-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/1d2ae14a4b18/sciadv.abm7947-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/569f26183f9c/sciadv.abm7947-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/b61104d60ae6/sciadv.abm7947-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/e69a386a5f8b/sciadv.abm7947-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/1d2ae14a4b18/sciadv.abm7947-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7795/9054011/569f26183f9c/sciadv.abm7947-f4.jpg

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本文引用的文献

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Global burden of 87 risk factors in 204 countries and territories, 1990-2019: a systematic analysis for the Global Burden of Disease Study 2019.204 个国家和地区 1990-2019 年 87 种风险因素的全球负担:2019 年全球疾病负担研究的系统分析。
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X-ray Computed Tomography for Flame-Structure Analysis of Laminar Premixed Flames.
用于层流预混火焰结构分析的X射线计算机断层扫描
Combust Flame. 2019 Feb;200:142-154. doi: 10.1016/j.combustflame.2018.11.015. Epub 2018 Nov 28.
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Appl Opt. 2016 Jun 10;55(17):4691-8. doi: 10.1364/AO.55.004691.
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Densitometry and temperature measurement of combustion gas by X-ray Compton scattering.利用X射线康普顿散射对燃烧气体进行密度测量和温度测量。
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