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软质多孔超声绝缘体的制备

Elaboration of soft porous ultrasound insulators.

作者信息

Poupart Romain, Lacour Thomas, Darnige Pablo, Poncelet Olivier, Aristégui Christophe, Voisin Thomas, Marre Samuel, Brunet Thomas, Mondain-Monval Olivier

机构信息

Univ. Bordeaux, CNRS, UMR 5031, Centre de Recherche Paul Pascal F-33600 Pessac France

Univ. Bordeaux, CNRS, Bordeaux INP, Arts-et-Métiers, UMR 5295, Institut de Mécanique et d'Ingénierie F-33405 Talence France.

出版信息

RSC Adv. 2020 Nov 17;10(68):41946-41953. doi: 10.1039/d0ra07269a. eCollection 2020 Nov 11.

DOI:10.1039/d0ra07269a
PMID:35516577
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9057957/
Abstract

A simple and easy way is proposed for the fabrication of a highly attenuating composite material for underwater acoustics. The approach involves the introduction of porous polymer beads into a polyurethane matrix. The porous beads are prepared through an emulsion-templating approach, and two different processes are used. The first one uses microfluidics to synthesize beads of controlled diameter and porosity. The control over the bead size allows the selection of the frequency range where the material exhibits the highest acoustic attenuation. The second one uses a double emulsion approach and allows for the production of much larger quantities of beads. Both approaches yield materials exhibiting much higher acoustic absorption than the one obtained using the most commonly used micro-balloon inclusion. We present both the synthesis procedures and the structural and acoustic characterizations of the beads and the final acoustic materials.

摘要

提出了一种简单易行的方法来制备用于水下声学的高衰减复合材料。该方法包括将多孔聚合物珠粒引入聚氨酯基体中。多孔珠粒通过乳液模板法制备,并使用了两种不同的工艺。第一种工艺使用微流体技术合成直径和孔隙率可控的珠粒。对珠粒尺寸的控制使得能够选择材料表现出最高声衰减的频率范围。第二种工艺使用双乳液法,能够生产大量的珠粒。两种方法制备的材料都比使用最常用的微球夹杂法得到的材料具有更高的吸声性能。我们展示了珠粒以及最终声学材料的合成过程、结构和声学表征。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/eb40264f8500/d0ra07269a-f8.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/aa86cd5db4b9/d0ra07269a-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/eb40264f8500/d0ra07269a-f8.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/45ec772465c8/d0ra07269a-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/67985f12c1ce/d0ra07269a-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/87f7b2fdae44/d0ra07269a-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/8d6b6f074ac1/d0ra07269a-f4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/6c6a6bffae06/d0ra07269a-f5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/c5c0a2cc5e65/d0ra07269a-f6.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/aa86cd5db4b9/d0ra07269a-f7.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/e693/9057957/eb40264f8500/d0ra07269a-f8.jpg

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本文引用的文献

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Critical Role of a Nanometer-Scale Microballoon Shell on Bulk Acoustic Properties of Doped Soft Matter.
Langmuir. 2020 Jun 2;36(21):5787-5792. doi: 10.1021/acs.langmuir.0c00497. Epub 2020 May 21.
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Diffusion-limited dissolution of calcium carbonate in a hydrogel.碳酸钙在水凝胶中的扩散限制溶解。
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Soft porous silicone rubbers with ultra-low sound speeds in acoustic metamaterials.具有超低声速的软质多孔硅橡胶声超材料。
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Tailoring of the porous structure of soft emulsion-templated polymer materials.软乳液模板聚合物材料的多孔结构的定制。
Soft Matter. 2016 Jun 21;12(23):5154-63. doi: 10.1039/c6sm00461j. Epub 2016 May 19.
6
Soft porous silicone rubbers as key elements for the realization of acoustic metamaterials.柔软多孔硅橡胶作为实现声学超材料的关键元素。
Langmuir. 2015 Mar 17;31(10):3215-21. doi: 10.1021/la504720f. Epub 2015 Mar 3.
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