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尼日利亚一个二手汽车零部件市场周边土壤和河流沉积物中重金属的含量、分布、生态及人体健康风险评估

Level, distribution, ecological, and human health risk assessment of heavy metals in soils and stream sediments around a used-automobile spare part market in Nigeria.

作者信息

Kolawole T O, Ajibade O M, Olajide-Kayode J O, Fomba K W

机构信息

Department of Geological Sciences, Osun State University, Osogbo, Nigeria.

Department of Earth Sciences, Olabisi Onabanjo University, Ago-Iwoye, Nigeria.

出版信息

Environ Geochem Health. 2023 May;45(5):1573-1598. doi: 10.1007/s10653-022-01283-z. Epub 2022 May 10.

DOI:10.1007/s10653-022-01283-z
PMID:35536448
Abstract

The aim of this research was to assess the distribution, sources, contamination status, ecological risk, and human health risk of heavy metals (HMs) in soil and sediments of a used-automobile spare part market in Nigeria. Forty-three (43) soil samples were collected within a spare part market section (SPMS-17 samples), market-residential section (MRES-10 samples), traffic section (TRAS-10 samples), and non-market residential section (NMRS- 6 samples). Fifteen (15) stream sediments were collected within and around SPMS. Based on average concentrations, HMs (As, Cd, Cr, Cu, Fe, Mo, Pb, and Zn) had their highest values in SPMS, and their minimum values were observed in NMRS. The high concentration was as a result of contributions from anthropogenic activities such as the direct discharge of used-lubricant oil, scrap metals, tire wear, and traffic emission in the environment. However, Al, Co, and Mn were derived from the geology of the area. The same trend was observed in the stream sediment section (STSS), except that in addition to Al, Co and Mn in soils, Cr was also sourced from geogenic activity. There were moderate to high enrichment/contamination factors of the anthropogenically sourced HMs, especially in the soil of SPMS, MRES, TRAS and stream sediments (STSS). Similarly, high potential ecological risk (Er) and ecological risks (RI) were observed for As, Pb, and Cd in SPMS and STSS, while these were moderate in MRES and TRAS. Assessment of health risks was within acceptable limit for most of the HMs in the different sections for both adults and children, except As, Cd, and Pb in SPMS and STSS, which were beyond the acceptable limit for children. The carcinogenic risk was within the acceptable limit.

摘要

本研究的目的是评估尼日利亚一个二手汽车零部件市场的土壤和沉积物中重金属的分布、来源、污染状况、生态风险和人类健康风险。在一个零部件市场区域(SPMS - 17个样本)、市场住宅区(MRES - 10个样本)、交通区域(TRAS - 10个样本)和非市场住宅区(NMRS - 6个样本)内采集了43个土壤样本。在SPMS及其周边采集了15个河流沉积物样本。基于平均浓度,重金属(砷、镉、铬、铜、铁、钼、铅和锌)在SPMS中的含量最高,在NMRS中含量最低。高浓度是由于人为活动造成的,如废润滑油的直接排放、废金属、轮胎磨损以及环境中的交通排放。然而,铝、钴和锰来自该地区的地质情况。在河流沉积物区域(STSS)也观察到了相同的趋势,不同的是,除了土壤中的铝、钴和锰外,铬也是由地质活动产生的。人为来源的重金属存在中度到高度的富集/污染因素,特别是在SPMS、MRES、TRAS的土壤和河流沉积物(STSS)中。同样,在SPMS和STSS中,砷、铅和镉存在高潜在生态风险(Er)和生态风险指数(RI),而在MRES和TRAS中这些风险为中度。对不同区域的大多数重金属而言,成人和儿童的健康风险评估均在可接受范围内,但SPMS和STSS中的砷、镉和铅除外,这几种重金属对儿童而言超出了可接受范围。致癌风险在可接受范围内。

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