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新型添加型生物缓释碳源的制备及可行性研究。

Study on the preparation and feasibility of a novel adding-type biological slow-release carbon source.

机构信息

College of Environmental Science and Engineering, Taiyuan University of Technology, Taiyuan, 030024, PR China.

College of Environmental Science and Engineering, Taiyuan University of Technology, Taiyuan, 030024, PR China.

出版信息

J Environ Manage. 2022 Aug 15;316:115236. doi: 10.1016/j.jenvman.2022.115236. Epub 2022 May 11.

Abstract

The development of slow-release carbon sources is an effective biological treatment to remove nutrients from wastewater with low carbon-to-nitrogen ratio (C/N). Most filling-type slow-release carbon could not fulfil the needs of current wastewater treatment plants (WWTPs) process. And most adding-type slow-release carbon sources were prepared using some expensive chemical materials. In this study, combining the advantages of the aforementioned types, a novel adding-type wastepaper-flora (AT-WF) slow-release carbon source was proposed, aiming to realise wastepaper recycling in WWTPs. The screening and identification of the mixed flora, AT-WF carbon source release behaviour, and denitrification performance were investigated. The results showed that through the proposed screening method, a considerable proportion of cellulose-degradation-related genera was enriched, and the cellulose degradation ability and ratio of readily available carbon sources of flora T4, S4 and S5 were effectively strengthened. AT-WF had significant carbon release ability and stability, with an average total organic carbon (TOC) release of 8.82 ± 2.36 mg/g. Kinetic analysis showed that the entire carbon release process was more consistent with the first-order equation. Piecewise fitting with the Ritger-Peppas equation exhibited that the rapid-release (RR) stage was skeleton dissolution and the slow-release (SR) stage was Fick diffusion. Denitrification efficiency can achieve a high average removal efficiency of 94.17%, which could theoretically contribute 11.2% more to the total inorganic nitrogen (TIN) removal. Thus, this study indicated that AT-WF could be utilised as an alternative carbon source in WWTPs.

摘要

开发缓释碳源是一种有效的生物处理方法,可以去除低碳氮比(C/N)废水中的营养物质。大多数填充型缓释碳源无法满足当前污水处理厂(WWTP)的需求。大多数添加型缓释碳源是使用一些昂贵的化学材料制备的。在这项研究中,结合上述两种类型的优点,提出了一种新型的添加型废纸-菌群(AT-WF)缓释碳源,旨在实现 WWTP 中的废纸回收利用。考察了混合菌群的筛选与鉴定、AT-WF 碳源释放行为和反硝化性能。结果表明,通过提出的筛选方法,富集了相当比例的纤维素降解相关属,有效增强了菌群 T4、S4 和 S5 的纤维素降解能力和易利用碳源比例。AT-WF 具有显著的碳释放能力和稳定性,平均总有机碳(TOC)释放量为 8.82±2.36mg/g。动力学分析表明,整个碳释放过程更符合一级方程。用 Ritger-Peppas 方程分段拟合表明,快速释放(RR)阶段是骨架溶解,缓慢释放(SR)阶段是菲克扩散。反硝化效率可达到 94.17%的平均去除效率,理论上可为总无机氮(TIN)去除贡献 11.2%以上。因此,本研究表明 AT-WF 可作为 WWTP 的替代碳源。

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