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超快激光诱导垂直磁各向异性抑制实现的CoFeB/MgO/CoFeB隧道结中的自旋重取向转变

Spin reorientation transition in CoFeB/MgO/CoFeB tunnel junction enabled by ultrafast laser-induced suppression of perpendicular magnetic anisotropy.

作者信息

Shelukhin Leonid A, Gareev Rashid R, Zbarsky Vladyslav, Walowski Jakob, Münzenberg Markus, Pertsev Nikolay A, Kalashnikova Alexandra M

机构信息

Ioffe Institute, 194021 St. Petersburg, Russia.

Institute of Experimental and Applied Physics, University of Regensburg, 93040 Regensburg, Germany.

出版信息

Nanoscale. 2022 Jun 9;14(22):8153-8162. doi: 10.1039/d2nr00637e.

Abstract

Magnetic tunnel junction (MTJ) is a leading contender for next generation high-density nonvolatile memory technology. Fast and efficient switching of MTJs between different resistance states is a challenging problem, which can be tackled by using an unconventional stimulus-a femtosecond laser pulse. Herein, we report an experimental study of the laser-induced magnetization dynamics in a CoFeB/MgO/CoFeB (CoFeB/MgO/CoFeB) MTJ with ultrathin CoFeB electrodes possessing perpendicular magnetic anisotropy (PMA). In addition to ultrafast demagnetization, a femtosecond laser pulse gives rise to a decaying magnetization precession in the thinner CoFeB layer subjected to an in-plane magnetic field, while the magnetization of the thicker CoFeB layer remains aligned with the applied field. Remarkably, the precession frequency demonstrates a strong and nonlinear rise with increasing pump fluence, which stems from the complete laser-induced suppression of PMA in the 1.2 nm-thick CoFeB electrode reached at a moderate fluence of about 1.8 mJ cm at room temperature. This important feature signifies that the laser excitation of such an electrode can enable an ultrafast transition from a perpendicular-to-plane to an in-plane magnetization orientation in the absence of a magnetic field and reveals the feasibility of the laser-driven switching of MTJ between different states. The revealed gradual quenching of PMA with increasing fluence is explained by the laser-induced heating of the MTJ, which affects the interfacial magnetic anisotropy stronger than the shape anisotropy. Interestingly, at low fluences, the values of interfacial anisotropy and saturation magnetization altered by the laser excitation scale with each other as expected for the two-site anisotropic exchange interaction, but the scaling exponent increases significantly at moderate fluences, which enables the realization of a laser-induced spin reorientation transition.

摘要

磁性隧道结(MTJ)是下一代高密度非易失性存储技术的主要竞争者。在不同电阻状态之间快速高效地切换MTJ是一个具有挑战性的问题,可以通过使用一种非常规刺激——飞秒激光脉冲来解决。在此,我们报告了对具有垂直磁各向异性(PMA)的超薄CoFeB电极的CoFeB/MgO/CoFeB(CoFeB/MgO/CoFeB)MTJ中激光诱导的磁化动力学的实验研究。除了超快退磁外,飞秒激光脉冲还会在受到面内磁场作用的较薄CoFeB层中引起磁化的衰减进动,而较厚CoFeB层的磁化则保持与外加磁场对齐。值得注意的是,进动频率随着泵浦能量密度的增加呈现出强烈的非线性上升,这源于在室温下约1.8 mJ/cm²的中等能量密度下,1.2 nm厚的CoFeB电极中激光诱导的PMA完全被抑制。这一重要特征表明,对这种电极进行激光激发能够在没有磁场的情况下实现从垂直磁化到面内磁化取向的超快转变,并揭示了激光驱动MTJ在不同状态之间切换的可行性。随着能量密度增加,PMA逐渐淬灭是由激光诱导的MTJ加热所解释的,这种加热对界面磁各向异性的影响比对形状各向异性的影响更强。有趣的是,在低能量密度下,激光激发改变的界面各向异性值和饱和磁化强度彼此按预期的双位点各向异性交换相互作用进行缩放,但在中等能量密度下,缩放指数显著增加,这使得能够实现激光诱导的自旋重取向转变。

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