用于高效光催化析氢的二维共价有机框架
2D Covalent Organic Frameworks Toward Efficient Photocatalytic Hydrogen Evolution.
作者信息
Li Yang, Song Xiaoyu, Zhang Guang, Wang Lei, Liu Yi, Chen Weihua, Chen Long
机构信息
Shenzhen Key Laboratory of Polymer Science and Technology, Guangdong Research Center for Interfacial Engineering of Functional Materials, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518060, P. R. China.
College of Physics and Optoelectronic Engineering, Shenzhen University, Shenzhen, 518060, P. R. China.
出版信息
ChemSusChem. 2022 Aug 5;15(15):e202200901. doi: 10.1002/cssc.202200901. Epub 2022 Jun 22.
Efficiently producing clean energy is of great importance for sustainable development of the environment. Solar-driven water splitting for H evolution has an important role among the renewable energy technologies. Developing high-performance and cost-effective photocatalysts is still a critical task before practical application. 2D Covalent organic frameworks (COFs) as photocatalysts have recently attracted widespread interest thanks to their tunable optical bandgaps, tailor-made functionality, excellent crystallinity, high specific surface area, and good photo- and chemical stability. This Review focuses on the representative progress and remaining challenges in 2D COF-based photocatalysts for hydrogen evolution.
高效生产清洁能源对于环境的可持续发展至关重要。太阳能驱动水分解制氢在可再生能源技术中具有重要作用。在实际应用之前，开发高性能且具有成本效益的光催化剂仍然是一项关键任务。二维共价有机框架（COF）作为光催化剂，由于其可调谐的光学带隙、定制的功能、优异的结晶度、高比表面积以及良好的光稳定性和化学稳定性，最近引起了广泛关注。本综述重点介绍了基于二维COF的析氢光催化剂的代表性进展和 remaining challenges。 （注：原文中“remaining challenges”未翻译，可能是原文有误，推测可能是“remaining challenges”应改为“remaining challenges”，直译为“剩余挑战”，意译为“现存挑战”等，此处按原文呈现）
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