College of Geography and Environmental Sciences, Zhejiang Normal University, Jinhua 321004, China.
Int J Environ Res Public Health. 2022 Jun 9;19(12):7091. doi: 10.3390/ijerph19127091.
Source apportionment of PM in Lanzhou, China, was carried out using positive matrix factorization (PMF). Seventeen elements (Ca, Fe, K, Ti, Ba, Mn, Sr, Cd, Se, Pb, Cu, Zn, As, Ni, Co, Cr, V), water-soluble ions (Na, NH, K, Mg, Ca, Cl, NO, SO), and organic carbon (OC) and elemental carbon (EC) were analyzed. The results indicated that the mean concentration of PM was 178.63 ± 96.99 μg/m. In winter, the PM concentration was higher during the day than at night, and the opposite was the case in summer, and the nighttime PM concentration was 1.3 times higher than during the day. Water-soluble ions were the dominant component of PM during the study. PMF source analysis revealed six sources in winter, during the day and night: salt lakes, coal combustion, vehicle emissions, secondary aerosols, soil dust, and industrial emissions. In summer, eight sources during the day and night were identified: soil dust, coal combustion, industrial emissions, vehicle emissions, secondary sulfate, salt lakes, secondary aerosols, and biomass burning. Secondary aerosols, coal combustion, and vehicle emissions were the dominant sources of PM. In winter, the proportions of secondary aerosols and soil dust sources were greater during the day than at night, and the opposite was the case in summer. The coal source, industrial emissions source, and motor vehicle emissions source were greater at night than during the day in winter. This work can serve as a case study for further in-depth research on PM pollution and source apportionment in Lanzhou, China.
在中国兰州,采用正定矩阵因子分析(PMF)对 PM 进行了源解析。分析了 17 种元素(Ca、Fe、K、Ti、Ba、Mn、Sr、Cd、Se、Pb、Cu、Zn、As、Ni、Co、Cr、V)、水溶性离子(Na、NH、K、Mg、Ca、Cl、NO、SO)、有机碳(OC)和元素碳(EC)。结果表明,PM 的平均浓度为 178.63±96.99μg/m。在冬季,白天的 PM 浓度高于夜间,而夏季则相反,夜间的 PM 浓度是白天的 1.3 倍。在研究期间,水溶性离子是 PM 的主要成分。PMF 源分析显示,冬季白天和夜间有 6 个污染源:盐湖、煤炭燃烧、车辆排放、二次气溶胶、土壤尘和工业排放。在夏季,白天和夜间共识别出 8 个污染源:土壤尘、煤炭燃烧、工业排放、车辆排放、二次硫酸盐、盐湖、二次气溶胶和生物质燃烧。二次气溶胶、煤炭燃烧和车辆排放是 PM 的主要来源。在冬季,白天二次气溶胶和土壤尘的比例大于夜间,而夏季则相反。在冬季,煤炭、工业排放和机动车排放源在夜间大于白天。这项工作可以作为兰州 PM 污染和源解析进一步深入研究的案例。