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通过半解析模型校准费米速度以探索石墨烯纳米带阵列的等离激元特性

Calibration of Fermi Velocity to Explore the Plasmonic Character of Graphene Nanoribbon Arrays by a Semi-Analytical Model.

作者信息

Tene Talia, Guevara Marco, Viteri Edwin, Maldonado Alba, Pisarra Michele, Sindona Antonello, Vacacela Gomez Cristian, Bellucci Stefano

机构信息

Departamento de Química, Universidad Técnica Particular de Loja, Loja 110160, Ecuador.

School of Physical Sciences and Nanotechnology, Yachay Tech University, Urcuquí 100119, Ecuador.

出版信息

Nanomaterials (Basel). 2022 Jun 13;12(12):2028. doi: 10.3390/nano12122028.

Abstract

We present an analysis of the electronic and plasmonic behavior of periodic planar distributions of sufficiently wide graphene nanoribbons, for which a thorough ab initio investigation is practically unfeasible. Our approach is based on a semi-analytical model whose only free parameter is the charge carrier velocity, which we estimate by density-functional theory calculations on graphene. By this approach, we show that the plasmon resonance energies of the scrutinized systems fall in the lower THz band, relevant for optoelectronic and photonic applications. We further observe that these energies critically depend on the charge carrier concentration, ribbon width, electron relaxation rate, and in-plane transferred momentum angle, thus, suggesting a tunability of the associated light-matter modes.

摘要

我们对足够宽的石墨烯纳米带的周期性平面分布的电子和等离子体行为进行了分析,对于这种分布,进行全面的从头算研究实际上是不可行的。我们的方法基于一个半解析模型,其唯一的自由参数是电荷载流子速度,我们通过对石墨烯的密度泛函理论计算来估计该速度。通过这种方法,我们表明所研究系统的等离子体共振能量落在较低的太赫兹频段,这与光电和光子应用相关。我们进一步观察到,这些能量关键取决于电荷载流子浓度、带宽度、电子弛豫率和面内转移动量角,因此表明相关的光与物质模式具有可调性。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8297/9229183/802eaceb40a3/nanomaterials-12-02028-g001.jpg

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