Zhang Shihui, Sun Xinghua, Liu Naidi, Mi Jing
College of Information Science and Engineering, Hebei North University, Zhangjiakou, Hebei 075000, China.
Int J Anal Chem. 2022 Jun 17;2022:7207020. doi: 10.1155/2022/7207020. eCollection 2022.
In order to solve the problem that atmospheric particulate matter has become the primary pollutant with serious harm and complex sources in recent years, this paper proposes an accurate identification method of pollution sources based on a receptor model to obtain the contribution rate of each pollution source category. This method takes the 75-day measured environmental receptor data of an area under the artificial intelligence cloud model as the basic data, uses the normrnd () function to expand the receptor data, and uses the positive definite matrix factor analysis (PMF) and principal component analysis (PCA) models to verify the rationality of the data expansion. The results are as follows: the number of extended simulated receptor component spectra has a certain effect on the PCA analysis results, but the effect is smaller than the extended range. All relative errors are less than 14%, and the relative error is the smallest when the six simulated receptor component spectra are expanded, that is, the PCA analysis results of the expanded data are most consistent with the measured data; the number of expanded simulated receptor component spectra has a certain influence on the PMF analysis results. But the relative error is less than 40%. When extending the spectrum of six simulated receptor components, the relative error is the smallest, that is, the PMF analysis results of the extended data are most consistent with the measured data. It is proven that this method provides a more direct basis for the targeted treatment of pollution sources that are more harmful to human health.
为解决近年来大气颗粒物已成为危害严重、来源复杂的首要污染物这一问题,本文提出一种基于受体模型的污染源精准识别方法,以获取各污染源类别的贡献率。该方法以人工智能云模型下某区域75天的实测环境受体数据为基础数据,利用normrnd()函数对受体数据进行扩展,并采用正定矩阵因子分析(PMF)和主成分分析(PCA)模型验证数据扩展的合理性。结果表明:扩展模拟受体组分谱数量对PCA分析结果有一定影响,但影响小于扩展范围。所有相对误差均小于14%,当扩展6个模拟受体组分谱时相对误差最小,即扩展后数据的PCA分析结果与实测数据最吻合;扩展模拟受体组分谱数量对PMF分析结果有一定影响,但相对误差小于40%。当扩展6个模拟受体组分谱时相对误差最小,即扩展后数据的PMF分析结果与实测数据最吻合。证明该方法为针对性治理对人体健康危害更大的污染源提供了更直接的依据。