Monsoon climate controls metal loading in global hotspot region of transboundary air pollution.

Eastern Asia is a major source of global air pollution. The distribution and intensity of these emissions are becoming well characterized, but their impact on the earth surface considering regional hydroclimatological settings has yet to be quantified. Here we show high-resolution spatiotemporal trace metal distributions of precipitation samples collected throughout the Japanese archipelago in 2013, when the world's coal consumption was the greatest, to depict the mass transportation and deposition of pollution. The results show that metals emitted through coal combustion transported from the continent via prevailing wind were intensively deposited along the western coast of the archipelago during winter due to heavy snowing, resulting in lead (Pb) concentration of precipitations exceed the critical level (> 10 μg l). About 1497 tons of Pb of continental origin loaded through wet deposition accounted for over ca. 87% of the total annual flux in 2013, which constituted ca. 18.5% of the total emissions from China in 2012. This study presents the first detailed picture of monsoon climate-controlled atmospheric metal transportation and loading in the hotspot region after the phase-out of leaded gasoline in the twentieth century. The dataset can serve as a base for evaluating the effect of countermeasures implemented recent year.