Geology Department, Middlebury College, Middlebury, VT 05753, USA.
Sci Total Environ. 2022 Oct 20;844:156999. doi: 10.1016/j.scitotenv.2022.156999. Epub 2022 Jun 28.
Mineral dust was collected with a network of passive samplers in the Uinta Mountains (Utah, USA) over a 10-year period to evaluate the relation between regional drought and dust deposition. A total of 72 samples from eight collectors were analyzed for flux, grain size distribution, mineralogy, geochemistry, and their Sr and Nd isotopic fingerprint. The dust is primarily very fine silt, with an average median grain size of 11.6 μm. The clay minerals illite and kaolinite are common in the dust, along with quartz, potassium feldspar, and plagioclase. The most abundant elements (after Si) are Al > Fe > K > Ca > Mg > Ti. The trace elements Cd, Sn, Sb, Zn, Cu, As, and Pb are present at abundances greatly in excess of normal levels in upper crustal rocks. Dust fluxes average 14.4 mg/m/day, generally decrease at higher elevations and toward the eastern end of the range, and are significantly higher in summer. Annual fluxes range from 1.4 to 5.8 g/m/yr with a decadal average of 3.4 g/m/yr. Rates of dust deposition are significantly correlated with regional drought severity from the Standardized Precipitation-Evapotranspiration Index (SPEI) for the southwestern US over 2, 3, and 6-month time scales. Previous work has demonstrated a connection between drought in the southwestern US and the abundance of fine (PM) material aloft. This work is the first to use long-term monitoring of annual dust deposition to confirm that the flux of silt-sized dust to mountain ecosystems is significantly correlated with regional drought severity.
在过去的 10 年中,美国犹他州的尤因塔山脉(Uinta Mountains)使用被动采样器网络收集了矿物质尘埃,以评估区域干旱与尘埃沉积之间的关系。对来自八个收集器的 72 个样本进行了通量、粒度分布、矿物学、地球化学以及 Sr 和 Nd 同位素指纹分析。尘埃主要为非常细的粉砂,平均中值粒径为 11.6μm。尘埃中常见的粘土矿物有伊利石和高岭石,还有石英、钾长石和斜长石。最丰富的元素(除 Si 外)为 Al > Fe > K > Ca > Mg > Ti。痕量元素 Cd、Sn、Sb、Zn、Cu、As 和 Pb 的丰度大大超过了地壳岩石的正常水平。尘埃通量平均为 14.4mg/m/天,通常在较高海拔和山脉范围的东端降低,夏季明显升高。年通量范围为 1.4 至 5.8 g/m/yr,十年平均值为 3.4 g/m/yr。尘埃沉积速率与美国西南部标准降水蒸散指数(SPEI)的区域干旱严重程度显著相关,该指数的时间尺度为 2、3 和 6 个月。之前的研究表明,美国西南部的干旱与高空细颗粒物(PM)物质的丰度之间存在联系。这项工作首次利用长期监测的年度尘埃沉积来证实,山区生态系统中细尘通量与区域干旱严重程度显著相关。