Xu Meng-Qi, Yang Wen-Tao, Yang Li-Yu, Chen Yong-Lin, Jing Hao-Nan, Wu Pan
College of Resources and Environmental Engineering, Guizhou University, Guiyang 550025, China.
Laboratory of Karst Georesources and Environment (Guizhou University), Ministry of Education, Guiyang 550025, China.
Huan Jing Ke Xue. 2022 Jul 8;43(7):3799-3810. doi: 10.13227/j.hjkx.202111053.
An extensive investigation of heavy metal (Cd, Hg, As, Pb, and Cr) levels in 137 pairs of soil-maize/rice samples was conducted in cultivated land from a typical karst mountain area in the Northwest of Guizhou Province. A health risk assessment model was used to assess the health risks of those areas, and the environmental benchmarks of heavy metals in soils were evaluated using the species sensitivity distribution (SSD) model. The results showed that the soils of maize and rice were polluted by heavy metals. Cd was the primary pollutant, with an exceeding rate ranging from 87% to 445%. The contaminated level of maize fields was higher than those of rice fields. In contrast, only 3.51% and 13.4% of Cd content in maize kernels and rice grains exceeded the national threshold, and the Cd heavy metal accumulation ability of rice was higher than that of maize. The carcinogenic and non-carcinogenic risks of heavy metals for adults and children in the study area were at a low level. The carcinogenic risk of rice consumption was slightly higher than that of maize, and the health risk to children was higher than that to adults. The results derived from the SSD method showed that the 95% and 5% hazardous concentrations (HC and HC) of maize fields were 0.67 for Cd, 771.99 for As, 40.85 for Pb and 609.88 for Cr mg·kg, and HCwere 48.47 for Cd, 159.67 for As, 1735.68 for Pb and 1671.74 for Cr mg·kg, respectively. The HC values of rice fields were 2.42 for Cd, 8.88 for As, 41.41 for Pb and 27.84 for Cr mg·kg, and the HC values were 48.47 for Cd, 159.67 for As, 1735.68 for Pb and 1671.74 for Cr mg·kg, respectively. The HC values of Cd, As, and Cr in maize fields and Cd in rice fields were significantly higher than the soil risk screening values in the current standard, and the HC values of the two fields were higher than the soil risk intervened values. The results indicated that the current standard would be too strict to evaluate the actual pollution level of soil heavy metals in this area.
对贵州省西北部典型喀斯特山区耕地中的137对土壤 - 玉米/水稻样本中的重金属(镉、汞、砷、铅和铬)含量进行了广泛调查。采用健康风险评估模型评估这些区域的健康风险,并使用物种敏感性分布(SSD)模型评估土壤中重金属的环境基准。结果表明,玉米和水稻土壤受到重金属污染。镉是主要污染物,超标率在87%至445%之间。玉米田的污染程度高于稻田。相比之下,玉米籽粒和稻谷中镉含量分别只有3.51%和13.4%超过国家阈值,且水稻对镉重金属的积累能力高于玉米。研究区域内重金属对成人和儿童的致癌和非致癌风险处于低水平。食用水稻的致癌风险略高于玉米,对儿童的健康风险高于成人。SSD方法得出的结果表明,玉米田镉、砷、铅和铬的95%和5%危险浓度(HC和HC)分别为0.67、771.99、40.85和609.88毫克·千克,HC分别为48.47、159.67、(此处原文可能有误,推测应为1735.68)和1671.74毫克·千克。稻田镉、砷、铅和铬的HC值分别为2.42、8.88、41.41和27.84毫克·千克,HC值分别为48.47、159.67、1735.68和1671.74毫克·千克。玉米田镉、砷和铬以及稻田镉的HC值显著高于现行标准中的土壤风险筛选值,两块田的HC值均高于土壤风险干预值。结果表明,现行标准过于严格,无法评估该地区土壤重金属的实际污染水平。