Luan Chaoran, Shen Qiu, Rowell Nelson, Zhang Meng, Chen Xiaoqin, Huang Wen, Yu Kui
Laboratory of Ethnopharmacology, Tissue-orientated Property of Chinese Medicine Key Laboratory of Sichuan Province, West China School of Medicine, West China Hospital, Sichuan University, Chengdu, Sichuan, 610065, P. R. China.
National Engineering Research Center for Biomaterials, College of Biomedical Engineering, Sichuan University, Chengdu, Sichuan, 610065, P. R. China.
Angew Chem Int Ed Engl. 2022 Aug 26;61(35):e202205784. doi: 10.1002/anie.202205784. Epub 2022 Jul 20.
The transformations of colloidal semiconductor magic-size clusters (MSCs) are expected to occur with only discrete, step-wise redshifts in optical absorption. Here, we challenge this assumption presenting a novel, conceptually different transformation, for which the redshift is continuous. In the room-temperature transformation from CdTe MSC-448 to MSC-488 (designated by the peak wavelengths in nanometer), the redshift of absorption monitored in situ displays distinctly continuous and/or step-wise behavior. Based on conclusive evidence provided by real-time experiments, the former transformation is apparently direct and intra-cluster with a relatively large energy barrier. The latter transformation is indirect and assisted by MSC precursor compounds (PCs). The former transformation follows the latter often, being predominant at a relatively high temperature. The present findings encourage a reconsideration of the absorption redshift reported previously for transformations of binary II-VI MSCs, together with the pathway associated without the increase of cluster mass.
胶体半导体魔法尺寸团簇(MSC)的转变预计只会在光吸收中出现离散的、逐步的红移。在此,我们对这一假设提出挑战,展示了一种新颖的、概念上不同的转变,其红移是连续的。在从CdTe MSC - 448到MSC - 488的室温转变(由纳米级的峰值波长指定)中,原位监测的吸收红移表现出明显的连续和/或逐步行为。基于实时实验提供的确凿证据,前一种转变显然是直接的且发生在团簇内部,具有相对较大的能垒。后一种转变是间接的,并由MSC前体化合物(PC)辅助。前一种转变常常跟随后一种转变,在相对较高温度下占主导。目前的发现促使人们重新审视先前报道的二元II - VI MSC转变的吸收红移,以及与团簇质量增加无关的相关途径。