Department of Applied Physics, Stanford University, Stanford, California 94305, United States.
Department of Electrical Engineering, Stanford University, Stanford, California 94305, United States.
Nano Lett. 2022 Jul 27;22(14):5832-5840. doi: 10.1021/acs.nanolett.2c01579. Epub 2022 Jul 18.
We introduce and experimentally demonstrate electrically driven, spectrally selective thermal emitters based on globally aligned carbon nanotube metamaterials. The self-assembled metamaterial supports a high degree of nanotube ordering, enabling nanoscale ribbons patterned in the metamaterial to function both as Joule-heated incandescent filaments and as infrared hyperbolic resonators imparting spectral selectivity to the thermal radiation. Devices batch-fabricated on a single chip emit polarized thermal radiation with peak wavelengths dictated by their hyperbolic resonances, and their nanoscale heated dimensions yield modulation rates as high as 1 MHz. As a proof of concept, we show that two sets of thermal emitters on the same chip, operating with different peak wavelengths and modulation rates, can be used to sense carbon dioxide with one detector. We anticipate that the combination of batch fabrication, modulation bandwidth, and spectral tuning with chip-based nanotube thermal emitters will enable new modalities in multiplexed infrared sources.
我们介绍并实验演示了基于全局排列的碳纳米管超材料的电驱动、光谱选择热发射器。自组装的超材料支持高度的纳米管有序排列,使得在超材料中图案化的纳米级条带既可以作为焦耳加热的白炽灯丝,又可以作为红外双曲线谐振器,赋予热辐射光谱选择性。在单个芯片上批量制造的器件发射具有由其双曲线共振决定的峰值波长的偏振热辐射,并且它们的纳米级加热尺寸产生高达 1 MHz 的调制速率。作为概念验证,我们表明同一芯片上的两组热发射器,其工作峰值波长和调制速率不同,可以使用一个探测器来感测二氧化碳。我们预计,基于纳米管热发射器的批量制造、调制带宽和光谱调谐的结合将在多路复用红外光源中开辟新的模式。