Northwest Institute of Nuclear Technology, Xi'an 710024, China.
Department of Environmental and Resource Engineering, Technical University of Denmark, DTU Risø Campus, 4000 Roskilde, Denmark.
Molecules. 2022 Jul 15;27(14):4536. doi: 10.3390/molecules27144536.
The determination of Am in the environment is of importance in monitoring its release and assessing its environmental impact and radiological risk. This paper aims to give an overview about the recent developments and the state-of-art analytical methods for Am determination in environmental samples. Thorough discussions are given in this paper covering a wide range of aspects, including sample pre-treatment and pre-concentration methods, chemical separation techniques, source preparation, radiometric and mass spectrometric measurement techniques, speciation analyses, and tracer applications. The paper focuses on some hyphenated separation methods based on different chromatographic resins, which have been developed to achieve high analytical efficiency and sample throughput for the determination of Am. The performances of different radiometric and mass spectrometric measurement techniques for Am are evaluated and compared. Tracer applications of Am in the environment, including speciation analyses of Am, and applications in nuclear forensics are also discussed.
在环境中测定镅对于监测其释放以及评估其环境影响和辐射风险具有重要意义。本文旨在概述环境样品中镅测定的最新发展和分析方法。本文涵盖了广泛的方面,包括样品预处理和预浓缩方法、化学分离技术、源制备、放射性和质谱测量技术、形态分析和示踪剂应用。本文重点介绍了一些基于不同色谱树脂的联用分离方法,这些方法的发展旨在实现分析效率和样品通量的提高,以实现镅的测定。评估和比较了不同放射性和质谱测量技术对镅的性能。还讨论了镅在环境中的示踪剂应用,包括镅的形态分析和在核取证中的应用。