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先锋号,一台高分辨率单晶极化中子衍射仪。

PIONEER, a high-resolution single-crystal polarized neutron diffractometer.

作者信息

Liu Yaohua, Cao Huibo, Rosenkranz Stephan, Frost Matthew, Huegle Thomas, Lin Jiao Y Y, Torres Peter, Stoica Alexandru, Chakoumakos Bryan C

机构信息

Second Target Station, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA.

Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA.

出版信息

Rev Sci Instrum. 2022 Jul 1;93(7):073901. doi: 10.1063/5.0089524.

Abstract

PIONEER is a high Q-resolution, single-crystal, polarized neutron diffractometer at the Second Target Station (STS), Oak Ridge National Laboratory. It will provide the unprecedented capability of measuring tiny crystals (0.001 mm, i.e., x-ray diffraction size), ultra-thin films (10 nm thickness), and weak structural and magnetic transitions. PIONEER benefits from the increased peak brightness of STS cold-neutron sources and uses advanced Montel mirrors that are able to deliver a focused beam with a high brilliance transfer, a homogeneous profile, and a low background. Monte Carlo simulations suggest that the optimized instrument has a high theoretical peak brilliance of 2.9 × 10 n cm sr Å s at 2.5 Å at the sample position, within a 5 × 5 mm region and a ±0.3° divergence range. The moderator-to-sample distance is 60 m, providing a nominal wavelength band of 4.3 Å with a wavelength resolution better than 0.2% in the wavelength range of 1.0-6.0 Å. PIONEER is capable of characterizing large-scale periodic structures up to 200 Å. With a sample-to-detector distance of 0.8 m, PIONEER accommodates various sample environments, including low/high temperature, high pressure, and high magnetic/electric field. A large cylindrical detector array (4.0 sr) with a radial collimator is planned to suppress the background scattering from sample environments. Bottom detector banks provide an additional 0.4 sr coverage or can be removed if needed to accommodate special sample environments. We present virtual experimental results to demonstrate the scientific performance of PIONEER in measuring tiny samples.

摘要

先锋号是位于橡树岭国家实验室第二靶站(STS)的一台高Q分辨率、单晶、极化中子衍射仪。它将具备测量微小晶体(0.001毫米,即X射线衍射尺寸)、超薄膜(10纳米厚度)以及微弱结构和磁转变的前所未有的能力。先锋号受益于STS冷中子源峰值亮度的提高,并使用先进的蒙特尔镜,能够提供具有高亮度传输、均匀分布和低背景的聚焦光束。蒙特卡罗模拟表明,优化后的仪器在样品位置2.5埃处,在5×5毫米区域和±0.3°发散范围内,理论峰值亮度高达2.9×10⁹ n cm⁻² sr⁻¹ Å⁻¹ s⁻¹。慢化剂到样品的距离为60米,在1.0 - 6.0埃的波长范围内提供标称波长带为4.3埃,波长分辨率优于0.2%。先锋号能够表征高达200埃的大规模周期性结构。样品到探测器的距离为0.8米,先锋号可容纳各种样品环境,包括低温/高温、高压以及高磁场/电场。计划采用带有径向准直器的大型圆柱形探测器阵列(4.0 sr)来抑制来自样品环境的背景散射。底部探测器组提供额外的0.4 sr覆盖范围,或者可根据需要移除,以适应特殊的样品环境。我们展示虚拟实验结果,以证明先锋号在测量微小样品方面的科学性能。

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