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在c轴单轴应力下SrRuO的超导性。

The superconductivity of SrRuO under c-axis uniaxial stress.

作者信息

Jerzembeck Fabian, Røising Henrik S, Steppke Alexander, Rosner Helge, Sokolov Dmitry A, Kikugawa Naoki, Scaffidi Thomas, Simon Steven H, Mackenzie Andrew P, Hicks Clifford W

机构信息

Max Planck Institute for Chemical Physics of Solids, Nöthnitzer Str 40, 01187, Dresden, Germany.

Nordita, KTH Royal Institute of Technology and Stockholm University, Hannes Alfvéns väg 12, SE-106 91, Stockholm, Sweden.

出版信息

Nat Commun. 2022 Aug 6;13(1):4596. doi: 10.1038/s41467-022-32177-4.

DOI:10.1038/s41467-022-32177-4
PMID:35933412
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9357014/
Abstract

Applying in-plane uniaxial pressure to strongly correlated low-dimensional systems has been shown to tune the electronic structure dramatically. For example, the unconventional superconductor SrRuO can be tuned through a single Van Hove point, resulting in strong enhancement of both T and H. Out-of-plane (c axis) uniaxial pressure is expected to tune the quasi-two-dimensional structure even more strongly, by pushing it towards two Van Hove points simultaneously. Here, we achieve a record uniaxial stress of 3.2 GPa along the c axis of SrRuO. H increases, as expected for increasing density of states, but unexpectedly T falls. As a first attempt to explain this result, we present three-dimensional calculations in the weak interaction limit. We find that within the weak-coupling framework there is no single order parameter that can account for the contrasting effects of in-plane versus c-axis uniaxial stress, which makes this new result a strong constraint on theories of the superconductivity of SrRuO.

摘要

已证明,对强关联低维系统施加面内单轴压力会极大地调整其电子结构。例如,非常规超导体SrRuO可通过单个范霍夫点进行调整,从而使Tc和Hc都得到显著增强。预计面外(c轴)单轴压力会通过同时将准二维结构推向两个范霍夫点,从而更强烈地调整该结构。在此,我们在SrRuO的c轴方向上实现了3.2 GPa的创纪录单轴应力。正如态密度增加所预期的那样,Hc增加,但出乎意料的是Tc下降。作为解释这一结果的首次尝试,我们在弱相互作用极限下进行了三维计算。我们发现在弱耦合框架内,没有单一的序参量能够解释面内与c轴单轴应力的对比效应,这使得这一新结果对SrRuO超导理论构成了强有力的约束。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/69babb6fadba/41467_2022_32177_Fig9_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/a99a62234846/41467_2022_32177_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/7b4e11e62d46/41467_2022_32177_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/e806d503bf53/41467_2022_32177_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/2a4d8ac2a5da/41467_2022_32177_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/560b8bf058bc/41467_2022_32177_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/fce8bd66e020/41467_2022_32177_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/3fb85c2296a2/41467_2022_32177_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/77508a7f03e8/41467_2022_32177_Fig8_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/69babb6fadba/41467_2022_32177_Fig9_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/a99a62234846/41467_2022_32177_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/7b4e11e62d46/41467_2022_32177_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/e806d503bf53/41467_2022_32177_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/2a4d8ac2a5da/41467_2022_32177_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/560b8bf058bc/41467_2022_32177_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/fce8bd66e020/41467_2022_32177_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/3fb85c2296a2/41467_2022_32177_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/77508a7f03e8/41467_2022_32177_Fig8_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b66a/9357014/69babb6fadba/41467_2022_32177_Fig9_HTML.jpg

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本文引用的文献

1
Unsplit superconducting and time reversal symmetry breaking transitions in SrRuO under hydrostatic pressure and disorder.静水压力和无序条件下 SrRuO 中未分裂的超导和时间反演对称性破缺转变
Nat Commun. 2021 Jun 24;12(1):3920. doi: 10.1038/s41467-021-24176-8.
2
Evidence for even parity unconventional superconductivity in SrRuO.锶钌氧化物中偶数奇偶性非常规超导性的证据。
Proc Natl Acad Sci U S A. 2021 Jun 22;118(25). doi: 10.1073/pnas.2025313118.
3
High-sensitivity heat-capacity measurements on SrRuO under uniaxial pressure.在单轴压力下对SrRuO进行的高灵敏度热容量测量。
Proc Natl Acad Sci U S A. 2021 Mar 9;118(10). doi: 10.1073/pnas.2020492118.
4
Reduction of the Spin Susceptibility in the Superconducting State of Sr_{2}RuO_{4} Observed by Polarized Neutron Scattering.通过极化中子散射观测到的Sr₂RuO₄超导态自旋磁化率的降低
Phys Rev Lett. 2020 Nov 20;125(21):217004. doi: 10.1103/PhysRevLett.125.217004.
5
Momentum-resolved superconducting energy gaps of SrRuO from quasiparticle interference imaging.基于准粒子干涉成像的SrRuO的动量分辨超导能隙
Proc Natl Acad Sci U S A. 2020 Mar 10;117(10):5222-5227. doi: 10.1073/pnas.1916463117. Epub 2020 Feb 24.
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Knight Shift and Leading Superconducting Instability from Spin Fluctuations in Sr_{2}RuO_{4}.Sr_{2}RuO_{4}中自旋涨落引起的超导不稳定性的骑士跃变。
Phys Rev Lett. 2019 Dec 13;123(24):247001. doi: 10.1103/PhysRevLett.123.247001.
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Superconducting Symmetries of Sr_{2}RuO_{4} from First-Principles Electronic Structure.Sr_{2}RuO_{4} 的超导对称性:来自第一性原理电子结构的研究
Phys Rev Lett. 2019 Nov 22;123(21):217005. doi: 10.1103/PhysRevLett.123.217005.
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Constraints on the superconducting order parameter in SrRuO from oxygen-17 nuclear magnetic resonance.氧-17 核磁共振对 SrRuO 中超导序参量的限制。
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Piezoelectric-based uniaxial pressure cell with integrated force and displacement sensors.带有集成式力和位移传感器的基于压电的单轴压力传感器。
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Superelasticity and cryogenic linear shape memory effects of CaFeAs.CaFeAs的超弹性和低温线性形状记忆效应
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