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蒙古国乌兰巴托市西南部家庭室内 PM 中颗粒结合型多环芳烃(PAHs)的特征。

Characteristics of particle-bound polycyclic aromatic hydrocarbons (PAHs) in indoor PM of households in the Southwest part of Ulaanbaatar capital, Mongolia.

机构信息

Centre for Natural Sciences, University of Pannonia, Egyetem street 10, Veszprém, 8200, Hungary.

School of Veterinary Medicine, Mongolian University of Life Sciences, Khan-Uul District, 17042, Ulaanbaatar, Mongolia.

出版信息

Environ Monit Assess. 2022 Aug 11;194(9):665. doi: 10.1007/s10661-022-10297-0.

DOI:10.1007/s10661-022-10297-0
PMID:35951250
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC9372015/
Abstract

Air pollution, including PM concentration in Ulaanbaatar (capital of Mongolia) is a serious matter of concern. As the majority of households use coal in large areas of the city, indoor air quality is also posing a serious risk to human health. This study investigated the concentration of polycyclic aromatic compounds (PAHs) in indoor particulate matter (PM) in 10 non-smoker households. Sampling was conducted in winter of 2018, between 27 January and 09 February. Concentrations of PM in the indoor air of households ranged between 62.8 and 324.8 µg m. Total concentration of PAHs also varied in a relatively wide range, between 46.2 and 175.7 ng m. Five-ring PAHs represented a considerably high fraction of total PAHs between 25 and 53%, benzo[b]fluoranthene (BbF) and benzo[a]pyrene (BaP) were the two predominant compounds within five-ring PAHs. Significant correlation was found between indoor and outdoor particulate matter levels in wintertime. Considering individual characteristic PAHs, heavier PAHs homologues (4- to 5-ring and 6-ring PAHs) were detected in all households, which suggested the influence of coal combustion and traffic exhaust. Health risk of children attributed to PAHs inhalation was assessed by taking into account the lifetime-average daily dose (LADD) and corresponding lifetime cancer risk. Lifetime average daily dose for children in only one household were slightly higher than health-based guideline level (1.0 × 10), defined by WHO, whereas LADD for adults and children of other households were within acceptable limit. The cancer risks from the exposure of children to air pollutants in all households except HH-3 were found high. In the Vibrio fischeri bioluminescence inhibition assay, according to the toxic unit (TU) values of indoor PM from ten households, all samples were classified as toxic.

摘要

空气污染,包括蒙古国乌兰巴托(首都)的 PM 浓度,是一个令人严重关切的问题。由于城市大部分地区的家庭大量使用煤炭,室内空气质量也对人类健康构成严重威胁。本研究调查了 10 户不吸烟家庭室内颗粒物(PM)中多环芳烃(PAHs)的浓度。采样于 2018 年冬季进行,时间为 1 月 27 日至 2 月 9 日。家庭室内空气中 PM 的浓度范围在 62.8 至 324.8µg/m3之间。室内空气中 PAHs 的总浓度也在相当大的范围内变化,在 46.2 至 175.7ng/m3之间。五环 PAHs 占总 PAHs 的相当大的比例,在 25%至 53%之间,苯并[b]荧蒽(BbF)和苯并[a]芘(BaP)是五环 PAHs 中的两种主要化合物。在冬季发现室内和室外颗粒物水平之间存在显著相关性。考虑到个体特征 PAHs,所有家庭都检测到较重的 PAHs 同系物(四环和五环及六环 PAHs),这表明煤炭燃烧和交通尾气的影响。通过考虑终生平均日剂量(LADD)和相应的终生癌症风险,评估了儿童因吸入 PAHs 而产生的健康风险。仅一户家庭中儿童的终生平均日剂量略高于世界卫生组织(WHO)定义的基于健康的指导水平(1.0×10),而其他家庭的成年人和儿童的 LADD 则在可接受范围内。除 HH-3 外,所有家庭儿童因暴露于空气污染物而面临的癌症风险都很高。在发光菌 Vibrio fischeri 生物发光抑制试验中,根据十个家庭室内 PM 的毒性单位(TU)值,所有样本均被归类为有毒。

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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9f71/9372015/e6d3228cd73c/10661_2022_10297_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9f71/9372015/af41f3ad8cac/10661_2022_10297_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9f71/9372015/192b9a79318c/10661_2022_10297_Fig7_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9f71/9372015/740e7ba72cc6/10661_2022_10297_Fig8_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9f71/9372015/1151fcf61ba3/10661_2022_10297_Fig9_HTML.jpg

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