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扭曲的WS/WS同质结构中莫尔激子的观测

Observation of moiré excitons in the twisted WS/WS homostructure.

作者信息

Wu Biao, Zheng Haihong, Li Shaofei, Ding Junnan, Zeng Yujia, Liu Zongwen, Liu Yanping

机构信息

School of Physics and Electronics, Hunan Key Laboratory for Super-Microstructure and Ultrafast Process, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, People's Republic of China.

State Key Laboratory of High-Performance Complex Manufacturing, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, People's Republic of China.

出版信息

Nanoscale. 2022 Sep 2;14(34):12447-12454. doi: 10.1039/d2nr02450k.

Abstract

Moiré superlattices offer a fascinating platform for designing the properties of optical excitons. The moiré pattern can generate an ordered exciton array in space, making it possible for topological excitons and quantum emitters. Recently, evidence of moiré excitons in the twisted heterostructures of TMDs has been widely reported. However, to date, the capture and investigation of moiré excitons in the twisted homostructure (T-HS) remain elusive. Here, we report the observation of moiré excitons in the WS/WS T-HS with a twist angle of about 1.5°. The PL spectrum of the T-HS region shows many small peaks with nearly constant peak spacing, which is attributed to the reconstructed moiré potential generated by the reconstructed moiré pattern to confine the intralayer excitons, thereby forming an ordered moiré exciton array. Furthermore, we have studied the influence of temperature and laser power on the moiré excitons as well as the valley polarization of the moiré excitons. Our results provide a promising prospect for further exploration of artificial excitonic crystals and quantum emitters of TMD moiré patterns.

摘要

莫尔超晶格为设计光学激子的性质提供了一个引人入胜的平台。莫尔图案可以在空间中产生有序的激子阵列,从而使拓扑激子和量子发射器成为可能。最近,在过渡金属二卤化物(TMDs)的扭曲异质结构中,莫尔激子的证据已被广泛报道。然而,迄今为止,在扭曲同质结构(T-HS)中捕获和研究莫尔激子仍然难以实现。在这里,我们报告了在扭曲角约为1.5°的WS/WS T-HS中观察到莫尔激子。T-HS区域的光致发光(PL)光谱显示出许多小峰,其峰间距几乎恒定,这归因于由重构的莫尔图案产生的重构莫尔势,以限制层内激子,从而形成有序的莫尔激子阵列。此外,我们研究了温度和激光功率对莫尔激子的影响以及莫尔激子的谷极化。我们的结果为进一步探索TMD莫尔图案的人工激子晶体和量子发射器提供了一个有前景的前景。

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